Performance of a proton exchange membrane fuel cell stack using conductive amorphous carbon-coated 304 stainless steel bipolar plates

被引:104
|
作者
Yi, Peiyun [1 ]
Peng, Linfa [1 ]
Feng, Lizhong [2 ]
Gan, Pin [2 ]
Lai, Xinmin [1 ]
机构
[1] Shanghai Jiao Tong Univ, State Key Lab Mech Syst & Vibrat, Shanghai 200240, Peoples R China
[2] SAIC Motor Corp Ltd, Shanghai 200041, Peoples R China
基金
中国国家自然科学基金;
关键词
Proton exchange membrane fuel cells; Bipolar plates; Amorphous carbon film; Stainless steel; Performance; GAS-DIFFUSION LAYER; STAINLESS-STEEL; CONTAMINATION; DEGRADATION; DURABILITY; MITIGATION; MECHANISMS; PEFC;
D O I
10.1016/j.jpowsour.2010.05.019
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In this study, 304 stainless steel (SS) bipolar plates are fabricated by flexible forming process and an amorphous carbon (a-C) film is coated by closed field unbalanced magnetron sputter ion plating (CFUBMSIP). The interfacial contact resistance (ICR), in-plane conductivity and surface energy of the a-C coated 304SS samples are investigated. The initial performance of the single cell with a-C coated bipolar plates is 923.9 mW cm(-2) at a cell voltage of 0.6 V, and the peak power density is 1150.6 mW cm(-2) at a current density of 2573.2 mA cm(-2). Performance comparison experiments between a-C coated and bare 304SS bipolar plates show that the single cell performance is greatly improved by the a-Ccoating. Lifetime test of the single cell over 200 h and contamination analysis of the tested membrane electrode assemble (M EA) indicate that the a-C coating has excellent chemical stability. A 100 W-class proton exchange membrane fuel cell (PEMFC) short stack with a-C coated bipolar plates is assembled and shows exciting initial performance. The stack also exhibits uniform voltage distribution, good short-term lifetime performance, and high volumetric power density and specific power. Therefore, a-C coated 304SS bipolar plates may be practically applied for commercialization of PEMFC technology. (C) 2010 Elsevier B.V. All rights reserved.
引用
收藏
页码:7061 / 7066
页数:6
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