A Highly Efficient Metal-Free Oxygen Reduction Electrocatalyst Assembled from Carbon Nanotubes and Graphene

被引:220
|
作者
Yang, Jia [1 ]
Sun, Haiyan [2 ]
Liang, Haiyi [1 ]
Ji, Hengxing [1 ]
Song, Li [1 ]
Gao, Chao [2 ]
Xu, Hangxun [1 ]
机构
[1] Univ Sci & Technol China, CAS Key Lab Soft Matter Chem, Dept Polymer Sci & Engn, Dept Modern Mech,Dept Mat Sci & Engn,Natl Synchro, Hefei 230026, Anhui, Peoples R China
[2] Zhejiang Univ, MOE Key Lab Macromol Synth & Functionalizat, Dept Polymer Sci & Engn, Hangzhou 310027, Zhejiang, Peoples R China
基金
中国国家自然科学基金;
关键词
HIGH-PERFORMANCE ELECTROCATALYSTS; DOPED CARBON; FREE CATALYSTS; NITROGEN; ALKALINE; IRON; NANOPLATELETS; POLYANILINE; DURABILITY; FRAMEWORKS;
D O I
10.1002/adma.201505855
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A novel carbon-nanotube-graphene hybrid nanostructure is developed using an aerosol-assisted assembly approach. After doping with nitrogen and phosphorus, the prepared hybrid nano materials exhibit excellent electrocatalytic performance for oxygen reduction in both alkaline and acidic media. This research presents a continuous and low-cost route to prepare high-performance metal-free electrocatalysts while replacing Pt-based materials.
引用
收藏
页码:4606 / 4613
页数:8
相关论文
共 50 条
  • [31] Three-Dimensional Nitrogen-Doped Carbon Nanotubes/Graphene Structure Used as a Metal-Free Electrocatalyst for the Oxygen Reduction Reaction
    Ma, Yanwen
    Sun, Liying
    Huang, Wen
    Zhang, Lingrong
    Zhao, Jin
    Fan, Quli
    Huang, Wei
    JOURNAL OF PHYSICAL CHEMISTRY C, 2011, 115 (50): : 24592 - 24597
  • [32] Nitrogen-Doped Porous Graphdiyne: A Highly Efficient Metal-Free Electrocatalyst for Oxygen Reduction Reaction
    Lv, Qing
    Si, Wenyan
    Yang, Ze
    Wang, Ning
    Tu, Zeyi
    Yi, Yuanping
    Huang, Changshui
    Jiang, Li
    Zhang, Mingjia
    He, Jianjiang
    Long, Yunze
    ACS APPLIED MATERIALS & INTERFACES, 2017, 9 (35) : 29744 - 29752
  • [33] Nitrogen-rich graphitic-carbon®graphene as a metal-free electrocatalyst for oxygen reduction reaction
    Begum, Halima
    Ahmed, Mohammad Shamsuddin
    Kim, Young-Bae
    SCIENTIFIC REPORTS, 2020, 10 (01)
  • [34] Nitrogen-rich graphitic-carbon@graphene as a metal-free electrocatalyst for oxygen reduction reaction
    Halima Begum
    Mohammad Shamsuddin Ahmed
    Young-Bae Kim
    Scientific Reports, 10
  • [35] Nitrogen-doped porous activated carbon derived from cocoon silk as a highly efficient metal-free electrocatalyst for the oxygen reduction reaction
    Fu, Peng
    Zhou, Lihua
    Sun, Lihua
    Huang, Baohua
    Yuan, Yong
    RSC ADVANCES, 2017, 7 (22) : 13383 - 13389
  • [36] Sulfur-containing carbon by flame synthesis as efficient metal-free electrocatalyst for oxygen reduction reaction
    Inamdar, Shaukatali
    Choi, Hyuck-Soo
    Wang, Peng
    Song, Min Young
    Yu, Jong-Sung
    ELECTROCHEMISTRY COMMUNICATIONS, 2013, 30 : 9 - 12
  • [37] Carbon-Doped Boron Nitride Nanosheet: An Efficient Metal-Free Electrocatalyst for the Oxygen Reduction Reaction
    Zhao, Jingxiang
    Chen, Zhongfang
    JOURNAL OF PHYSICAL CHEMISTRY C, 2015, 119 (47): : 26348 - 26354
  • [38] Simultaneous doping of nitrogen and fluorine into reduced graphene oxide: A highly active metal-free electrocatalyst for oxygen reduction
    Qiao, Xiaochang
    Liao, Shijun
    Wang, Guanghua
    Zheng, Ruiping
    Song, Huiyu
    Li, Xiuhua
    CARBON, 2016, 99 : 272 - 279
  • [39] A nitrogen and boron co-doped metal-free carbon electrocatalyst for an efficient oxygen reduction reaction
    Zhou, Yunjie
    Sun, Yue
    Wang, Huibo
    Zhu, Cheng
    Gao, Jin
    Wu, Dan
    Huang, Hui
    Liu, Yang
    Kang, Zhenhui
    INORGANIC CHEMISTRY FRONTIERS, 2018, 5 (11): : 2985 - 2991
  • [40] A study of defect-rich carbon spheres as a metal-free electrocatalyst for an efficient oxygen reduction reaction
    Xiang, Qin
    Yin, Wei
    Liu, Yuping
    Yu, Danmei
    Wang, Xiaoli
    Li, Sha
    Chen, Changguo
    JOURNAL OF MATERIALS CHEMISTRY A, 2017, 5 (46) : 24314 - 24320