Experimental and Quantum Chemical Approaches to Develop Highly Selective Nanocatalysts for CO2-free Power Circulation

被引：16

作者：

Yamauchi, Miho ^{[1
]}

Ozawa, Nobuki ^{[2
]}

Kubo, Momoji ^{[2
]}

机构：

[1] Kyushu Univ, Int Inst Carbon Neutral Energy Res WPI I2CNER, Nishi Ku, Motooka 744, Fukuoka 8190395, Japan

[2] Tohoku Univ, Inst Mat Res, Aoba Ku, 2-1-1 Katahira, Sendai, Miyagi 9808577, Japan

来源：

CHEMICAL RECORD | 2016年 / 16卷 / 05期

关键词：

carbon-neutral; density functional calculations; electrocatalysts; Fe-group nanoalloys; titanium; ETHYLENE-GLYCOL; HYDROGEN STORAGE; ELECTROCATALYTIC OXIDATION; STRUCTURAL TRANSFORMATION; ALLOY NANOPARTICLES; BIMETALLIC SURFACES; CATALYST; ELECTROOXIDATION; REDUCTION; METHANOL;

D O I：

10.1002/tcr.201600047

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Renewable electricity must be utilized to usefully suppress the atmospheric CO2 concentration and slow the progression of global warming. We have thus proposed a new concept involving CO2-free electric power circulation systems via highly selective electrochemical reactions of alcohol/carboxylic acid redox couples. Design concepts for nanocatalysts able to catalyze highly selective electrochemical reactions are provided from both experimental and quantum mechanical perspectives.

引用

页码：2249 / 2259

页数：11

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