Heat transfer and hydrogen permeability in modelling industrial membrane reactors for methane steam reforming

被引：64
|
作者：
De Falco, M. [1 ]
Di Paola, L. [1 ]
Marrelli, L. [1 ]
机构：
[1] Univ Roma La Sapienza, Dept Chem Engn, I-00184 Rome, Italy
来源：
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2007年 / 32卷 / 14期
关键词：
steam reforming; membrane reactor; heat transfer; hydrogen production;
D O I：
10.1016/j.ijhydene.2007.04.014
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
A non-isothermal, one-dimensional, pseudo-homogeneous model is used to simulate the behaviour of a fixed-bed membrane reactor for industrial production of hydrogen by steam reforming of methane. The attention is focused on the influence of heat transfer description on reactor performance: after a brief explanation of the physical meaning of coefficients used in heat transport from the reactor wall to the catalytic bed, several correlations are reported and tested. Reliable expressions of heat transfer coefficients, together with a precise knowledge of membrane permeability, are shown to be a basic requirement to get reliable results from reactor simulations. (c) 2007 International Association for Hydrogen Energy. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码：2902 / 2913
页数：12
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