Impact of wood combustion on indoor air quality

被引:37
|
作者
Vicente, E. D. [1 ]
Vicente, A. M. [1 ]
Evtyugina, M. [1 ]
Oduber, F. I. [2 ]
Amato, F. [3 ]
Querol, X. [3 ]
Alves, C. [1 ]
机构
[1] Univ Aveiro, Dept Environm & Planning, Ctr Environm & Marine Studies, P-3810193 Aveiro, Portugal
[2] Univ Leon, Dept Phys, IMARENAB, E-24071 Leon, Spain
[3] CSIC, Spanish Res Council, ID EA, Inst Environm Assessment & Water Res, Barcelona 08034, Spain
关键词
Mediterranean region; Indoor air quality; OC/EC; Organic markers; PM10; Residential biomass combustion; POLYCYCLIC AROMATIC-HYDROCARBONS; FINE-PARTICLE EMISSIONS; PARTICULATE MATTER CONCENTRATIONS; CHEMICAL-CHARACTERIZATION; ATMOSPHERIC AEROSOLS; SOURCE APPORTIONMENT; OPERATING-CONDITIONS; ELEMENTARY-SCHOOLS; GASEOUS EMISSIONS; MOLECULAR TRACERS;
D O I
10.1016/j.scitotenv.2019.135769
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The incomplete wood combustion in appliances operated in batch mode is a recognised source of both in- and outdoor airborne pollutants, especially particulate matter (PM). Data on pollutant levels and PM characteristics in households with wood burning devices in developed countries are scarce with most studies describing stove change out programmes or other intervention measures. The aim of the present study was to simultaneously evaluate indoor and outdoor concentrations of CO, CO2 and PM10 during the operation of wood burning appliances (open fireplace and woodstove) in unoccupied rural households. PM10 samples were analysed for water soluble inorganic ions, major and trace elements, organic carbon (OC), elemental carbon (EC), and detailed organic speciation. The CO 8-hour average concentrations did not exceed the protection limit despite the sharp increases observed in relation to background levels. During the open fireplace operation, PM10 levels rose up 12 times compared to background concentrations, while the airtight stove resulted in a 2-fold increase. The inhalation cancer risk of particulate bound PAHs in the room equipped with woodstove was estimated to be negligible while the long-term exposure to PAH levels measured in the fireplace room may contribute to the development of cancer. The excess lifetime cancer risk resulting from the partide-bound Cr(VI) exposure during the fireplace and woodstove operation was higher than 1.0 x 10(-6) and 1.0 x 10(-5), respectively. Levoglucosan was one of the most abundant individual species both indoors and outdoors. This study underlines air pollution hazards and risks arising from the operation of traditional wood burning appliances. (C) 2019 Elsevier B.V. All rights reserved.
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页数:17
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