Laser MBE growth of cobalt-platinum multilayers with perpendicular magnetic anisotropy

Periodic multilayers with perpendicular magnetic anisotropy (PMA) attract a lot of attention nowadays being fundamentally interesting from the point of view of interface magnetism. They also provide a suitable test bench for the studies of spatially resolved magnetization dynamics at picosecond time scale conducted at x-ray free electron laser (XFEL) facilities. In the present paper we have developed a novel laser molecular beam epitaxy (LMBE) approach to grow Co/Pt multilayers on crystalline Al2O3 (0001) substrates. By applying Kerr-effect magnetometry to the samples fabricated at different conditions, we have found it essential for the appearance of PMA, to perform metal deposition in 0.03 mbar of argon and to keep Co layer thickness below 4 angstrom. Along with magnetic studies, we have investigated crystal structure and depth resolved layer composition of the fabricated Co/Pt multilayers by applying electron diffraction, x-ray diffraction and x-ray reflectometry. The combined atomic-force/magnetic-force microscopy studies have revealed a very low surface roughness of down to 1 angstrom (for the samples grown at properly optimized growth conditions) and a pronounced labyrinth pattern of magnetic domains with a periodicity of 250 nm appropriate for XFEL studies of ultrafast optical magnetization. The presented LMBE approach to fabricate magnetically ordered heterostructures with a pronounced PMA is supposed to be an important milestone on the way of facilitating future design of nanomaterials for applications in magnetic memories and for fundamental studies of ultrafast magnetization dynamics.