Homogeneous nucleation in inhomogeneous media.: II.: Nucleation in a shear flow

被引：43

作者：

Reguera, D ^{[1
]}

Rubí, JM

机构：

[1] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA

[2] Norwegian Univ Sci & Technol, Dept Chem, N-7491 Trondheim, Norway

[3] Univ Barcelona, Dept Fis Fonamental, E-08028 Barcelona, Spain

来源：

JOURNAL OF CHEMICAL PHYSICS | 2003年 / 119卷 / 18期

关键词：

D O I：

10.1063/1.1614777

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We investigate the influence of a shear flow on the process of nucleation. Mesoscopic nonequilibrium thermodynamics is used to derive the Fokker-Planck equation governing the evolution of the cluster size distribution in a metastable phase subjected to a stationary flow. The presence of the flow manifests itself in the expression for the effective diffusion coefficient of a cluster and introduces modifications in the nucleation rate. The implications of these results in condensation and polymer crystallization are discussed. (C) 2003 American Institute of Physics.

引用

页码：9888 / 9893

页数：6

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