Coincidence imaging of polyatomic molecules via laser-induced Coulomb explosion

被引:34
|
作者
Gagnon, J. [1 ,2 ]
Lee, Kevin F. [2 ,3 ]
Rayner, D. M. [2 ]
Corkum, P. B. [1 ,2 ,3 ]
Bhardwaj, V. R. [1 ]
机构
[1] Univ Ottawa, Dept Phys, Ottawa, ON K1N 6N5, Canada
[2] Natl Res Council Canada, Steacie Inst Mol Sci, Ottawa, ON K1A 0R6, Canada
[3] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada
关键词
D O I
10.1088/0953-4075/41/21/215104
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We extend laser-induced Coulomb explosion imaging to retrieve the structure of the five-atom dichloromethane (CH2Cl2) molecule by developing coincidence imaging and geometry optimization techniques. By detecting all five atoms in coincidence, we show that, from the measured velocity vectors, the geometry of the molecules can be reconstructed.
引用
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页数:6
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