Facile fabrication of ordered mesoporous Bi/Ti-MCM-41 nanocomposites for visible light-driven photocatalytic degradation of methylene blue and CO oxidation

被引:25
|
作者
Mohamed, Shaimaa K. [1 ]
Ibrahim, Amr Awad [2 ,3 ]
Mousa, A. A. [1 ]
Betiha, Mohamed A. [4 ,5 ]
El-Sharkawy, E. A. [1 ]
Hassan, Hassan M. A. [1 ,5 ]
机构
[1] Suez Univ, Fac Sci, Dept Chem, Suez, Egypt
[2] Mansoura Univ, Fac Sci, Dept Chem, Mansoura, Egypt
[3] Virginia Commonwealth Univ, Dept Chem, Richmond, VA 23284 USA
[4] Egyptian Petr Res Inst, Cairo 11727, Egypt
[5] Cairo Univ, Egypt Nanotechnol Ctr EGNC, El Sheikh Zayed Campus, Giza 12588, Egypt
关键词
Mesoporous; Ti-MCM-41; Bi/Ti-MCM-41; composite; Carbon monoxide oxidation; Visible photocatalyst; TITANIA NANOPARTICLES; ROOM-TEMPERATURE; PHOTODEGRADATION; PERFORMANCE; PARTICLES; BENZENE; OXIDE; UV;
D O I
10.1016/j.seppur.2017.12.008
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Bi/Ti-MCM-41 nanocomposite was fabricated by a simple one-step impregnating approach. The composites have been exploited, for the first time, as a dual function catalyst for low-temperature CO oxidation under aerobic condition and a visible-light-driven photocatalyst for degradation of MB as organic pollutants. The promoting effect of bismuth species on Ti-MCM-41 has been investigated with the influence of introduced various Bi amount. It worth noting that the hexagonal mesostructured of Ti-MCM-41 remained unaltered and were not interrupted during the Bi deposition process. The bismuth species dispersed well and incorporated both within the mesochannel and the pore wall of Ti-MCM-41. The fabricated composite catalyst showed a significant catalytic performance compared to pristine Ti-MCM-41. The significant enhancement of the photodegradation performance of the Bi/Ti-MCM-41 composite could be assigned to the synergistic effects of interfaces between Bi2O3 species and TiO2. Therefore, the fabricated composite catalyst is a promising candidate for environmental applications.
引用
收藏
页码:174 / 183
页数:10
相关论文
共 46 条
  • [41] Fabrication and high photocatalytic performance of noble metal nanoparticles supported on 3DOM InVO4-BiVO4 for the visible-light-driven degradation of rhodamine B and methylene blue
    Ji, Kemeng
    Deng, Jiguang
    Zang, Hongjun
    Han, Jiuhui
    Arandiyan, Hamidreza
    Dai, Hongxing
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2015, 165 : 285 - 295
  • [42] Facile fabrication of fibrous Bi4Ti3O12/Bi2S3/MoS2with enhanced photocatalytic activities towards pollutant degradation under visible light irradiation
    Liu, Jun
    Hui, Qian
    Chang, Meng-Jie
    Cui, Wen-Na
    Xi, Tong
    Wang, Lin-Da
    Sun, Meng
    Yuan, Bin
    Ni, Fu-Rong
    JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2020, 31 (20) : 17688 - 17702
  • [43] Facile fabrication of fibrous Bi4Ti3O12/Bi2S3/MoS2 with enhanced photocatalytic activities towards pollutant degradation under visible light irradiation
    Jun Liu
    Qian Hui
    Meng-Jie Chang
    Wen-Na Cui
    Tong Xi
    Lin-Da Wang
    Meng Sun
    Bin Yuan
    Fu-Rong Ni
    Journal of Materials Science: Materials in Electronics, 2020, 31 : 17688 - 17702
  • [44] Facile fabrication of mesoporous BiOCl/(BiO)2CO3/Bi2O3 ternary flower-like heterostructured microspheres with high visible-light-driven photoactivity
    Etogo, Atangana
    Hu, Enlai
    Zhou, Chunmei
    Zhong, Yijun
    Hu, Yong
    Hong, Zhanglian
    JOURNAL OF MATERIALS CHEMISTRY A, 2015, 3 (44) : 22413 - 22420
  • [45] Synergistic effect of boron and sulphur co-doping g-C3N4 nanosheet/Ag2S heterojunctions for high-performance visible light-driven photocatalytic methylene blue
    Shanmugam, Paramasivam
    Parasuraman, Balaji
    Mandlimath, Triveni Rajashekhar
    Smith, Siwaporn Meejoo
    Thangavelu, Pazhanivel
    Tangjaideborisu, Yodchai
    Nakorn, Pariya Na
    Boonyuen, Supakorn
    INORGANIC CHEMISTRY COMMUNICATIONS, 2025, 174
  • [46] Highly efficient visible-light-driven photocatalytic degradation of VOCs by CO2-assisted synthesized mesoporous carbon confined mixed-phase TiO2 nanocomposites derived from MOFs
    Liu, Hongli
    Ma, Yaping
    Chen, Jiangyao
    Wen, Meicheng
    Li, Guiying
    An, Taicheng
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2019, 250 : 337 - 346