NaOH-embedded three-dimensional porous boron nitride for efficient formaldehyde removal

被引:17
|
作者
Li, Jie [1 ,2 ]
Jia, Huichao [1 ,2 ]
Ding, Yushi [3 ]
Luo, Han [1 ,2 ]
Abbas, Saleem [1 ,2 ]
Liu, Zhenya [1 ,2 ]
Hu, Long [1 ,2 ]
Tang, Chengchun [1 ,2 ]
机构
[1] Hebei Univ Technol, Sch Mat Sci & Engn, Tianjin 300130, Peoples R China
[2] Hebei Univ Technol, Hebei Key Lab Boron Nitride Micro & Nano Mat, Tianjin 300130, Peoples R China
[3] Cent China Normal Univ, Coll Chem, Wuhan 430079, Peoples R China
基金
中国国家自然科学基金;
关键词
three-dimensional porous boron nitride; NaOH-embeddment; formaldehyde adsorption; catalytic degradation; INDOOR AIR; ADSORPTION; OXIDATION; FABRICATION;
D O I
10.1088/0957-4484/26/47/475704
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Volatile organic compounds, especially formaldehyde (HCHO), are considered to be great sources of contaminants in indoor air. However, design and preparation of safe, cost-affordable, and reusable materials for HCHO removal at ambient conditions are still remarkably challenging. Here, we have developed a kind of novel NaOH-embedded three-dimensional porous boron nitride (NaOH-3D BN) with high and hierarchical porosities, which exhibit excellent removal performance for HCHO. The as-prepared 3D BN is used as an adsorbent and catalytic support, while the embedded NaOH is applied as a catalyst, giving rise to catalytic transformation from high-toxic HCHO to less-toxic formate and methoxy salts at room temperature. Furthermore, their effective reusability has been confirmed. Given the high removal and reusability performance as well as no use of precious materials, the NaOH-3D BN is envisaged to. be. valuable practically. for indoor air purification.
引用
收藏
页数:7
相关论文
共 50 条
  • [31] Condensation-assembly synthesis of three-dimensionally porous boron nitride for effective oil removal
    Yang S.
    Cao C.
    Yan S.
    Gu Y.
    Ji J.
    Zhou Z.
    Liu C.
    Yang J.
    Zhang R.
    Xue Y.
    Tang C.
    Chemosphere, 2023, 345
  • [32] Three-Dimensional Nanoporous Iron Nitride Film as an Efficient Electrocatalyst for Water Oxidation
    Yu, Fang
    Zhou, Haiqing
    Zhu, Zhuan
    Sun, Jingying
    He, Ran
    Bao, Jiming
    Chen, Shuo
    Ren, Zhifeng
    ACS CATALYSIS, 2017, 7 (03): : 2052 - 2057
  • [33] Design of Boron and Transition Metal Embedded Two-Dimensional Porous Carbon Nitride for Electrocatalytic Synthesis of Urea
    Cao, Xin
    Zhang, Dewei
    Gao, Yongqi
    Prezhdo, Oleg V.
    Xu, Lai
    JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2023, 146 (01) : 1042 - 1052
  • [34] Thermal conductivity and electrical properties of three-dimensional porous aluminum nitride/epoxy composites
    Wang X.
    Zhang C.
    Zhang T.
    Chi Q.
    Fuhe Cailiao Xuebao/Acta Materiae Compositae Sinica, 2023, 40 (06): : 3341 - 3349
  • [35] Porous graphitic carbon nitride nanosheets with three-dimensional interconnected network as electrode for supercapacitors
    Wang, Hui
    Liu, Yiwei
    Kong, Lirong
    Xu, Zhongyun
    Shen, Xiaoping
    Premlatha, Subramanian
    JOURNAL OF ENERGY STORAGE, 2023, 63
  • [36] Heteroatom nitrogen and oxygen co-doped three-dimensional honeycomb porous carbons for methylene blue efficient removal
    Zhuang, Qi-Qi
    Cao, Jing-Pei
    Wu, Yan
    Zhao, Ming
    Zhao, Xiao-Yan
    Zhao, Yun-Peng
    Bai, Hong-Cun
    APPLIED SURFACE SCIENCE, 2021, 546
  • [37] Three-dimensional porous adsorbent based on chitosan-alginate-cellulose sponge for selective and efficient removal of anionic dyes
    Wen, Zeng
    Gao, Die
    Niu, Hong
    Lin, Jing
    Li, Zhou
    Zeng, Jia
    Ke, Famin
    Zhang, Kailian
    Xia, Zhining
    Wang, Dandan
    JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2023, 11 (05):
  • [38] Constructing three-dimensional boron nitride network for highly thermally conductive epoxy resin composites
    Wu, Xian
    Liu, Wei
    Shi, Fa-guo
    Yang, Le
    Zhang, Chun
    POLYMER COMPOSITES, 2022, 43 (03) : 1711 - 1717
  • [39] Recent progress in thermally conductive polymer/boron nitride composites by constructing three-dimensional networks
    Bai, Xue
    Zhang, Chengxu
    Zeng, Xiaoliang
    Ren, Linlin
    Sun, Rong
    Xu, Jianbin
    COMPOSITES COMMUNICATIONS, 2021, 24
  • [40] Three-Dimensional Functionalized Boron Nitride Nanosheets/ZnO Superstructures for CO2 Capture
    Yang, Chen
    Liu, Dan
    Chen, Ying
    Chen, Cheng
    Wang, Jiemin
    Fan, Ye
    Huang, Shaoming
    Lei, Weiwei
    ACS APPLIED MATERIALS & INTERFACES, 2019, 11 (10) : 10276 - 10282