Severe haze in northern China: A synergy of anthropogenic emissions and atmospheric processes

被引:697
|
作者
An, Zhisheng [1 ,2 ,3 ,4 ,5 ]
Huang, Ru-Jin [1 ,2 ,3 ,4 ,5 ]
Zhang, Renyi [6 ,7 ]
Tie, Xuexi [1 ,3 ]
Li, Guohui [1 ,2 ,3 ]
Cao, Junji [1 ,2 ,3 ]
Zhou, Weijian [1 ,2 ,4 ,5 ]
Shi, Zhengguo [1 ,2 ,8 ]
Han, Yongming [1 ,2 ,3 ,8 ]
Gu, Zhaolin [8 ]
Ji, Yuemeng [6 ,9 ]
机构
[1] Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Shaanxi, Peoples R China
[2] Chinese Acad Sci, Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China
[3] Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian 710061, Shaanxi, Peoples R China
[4] Beijing Normal Univ, Interdisciplinary Res Ctr Earth Sci Frontier, Beijing 100875, Peoples R China
[5] Pilot Natl Lab Marine Sci & Technol Qingdao, Open Studio Ocean Continental Climate & Environm, Qingdao 266061, Peoples R China
[6] Texas A&M Univ, Dept Atmospher Sci, College Stn, TX 77843 USA
[7] Texas A&M Univ, Dept Chem, College Stn, TX 77843 USA
[8] Xi An Jiao Tong Univ, Dept Earth & Environm Sci, Xian 710049, Shaanxi, Peoples R China
[9] Guangdong Univ Technol, Sch Environm Sci & Engn, Guangzhou Key Lab Environm Catalysis & Pollut Con, Guangzhou 510006, Guangdong, Peoples R China
基金
中国国家自然科学基金;
关键词
severe haze; synergetic effects; anthropogenic emission; atmospheric chemistry; climate change; TIME CHEMICAL-CHARACTERIZATION; AIR-POLLUTANT EMISSIONS; FINE PARTICULATE MATTER; ASIAN SUMMER MONSOON; PARTICLE FORMATION; REGIONAL TRANSPORT; BOUNDARY-LAYER; BLACK CARBON; HEAVY HAZE; AEROSOL COMPOSITION;
D O I
10.1073/pnas.1900125116
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Regional severe haze represents an enormous environmental problem in China, influencing air quality, human health, ecosystem, weather, and climate. These extremes are characterized by exceedingly high concentrations of fine particulate matter (smaller than 2.5 mu m, or PM2.5) and occur with extensive temporal (on a daily, weekly, to monthly timescale) and spatial (over a million square kilometers) coverage. Although significant advances have been made in field measurements, model simulations, and laboratory experiments for fine PM over recent years, the causes for severe haze formation have not yet to be systematically/comprehensively evaluated. This review provides a synthetic synopsis of recent advances in understanding the fundamental mechanisms of severe haze formation in northern China, focusing on emission sources, chemical formation and transformation, and meteorological and climatic conditions. In particular, we highlight the synergetic effects from the interactions between anthropogenic emissions and atmospheric processes. Current challenges and future research directions to improve the understanding of severe haze pollution as well as plausible regulatory implications on a scientific basis are also discussed.
引用
收藏
页码:8657 / 8666
页数:10
相关论文
共 50 条
  • [41] Hydrochemistry characters and hydrochemical processes under the impact of anthropogenic activity in the Yiyuan city, Northern China
    Zhenyan Wang
    Zongjun Gao
    Shu Wang
    Jiutan Liu
    Wei Li
    Qijun Deng
    Lin Lv
    Yuanqing Liu
    Qiao Su
    Environmental Earth Sciences, 2021, 80
  • [42] European emissions of atmospheric mercury from anthropogenic sources in 1995
    Pacyna, EG
    Pacyna, JM
    Pirrone, N
    ATMOSPHERIC ENVIRONMENT, 2001, 35 (17) : 2987 - 2996
  • [43] Unraveling the dynamics of atmospheric methane: the impact of anthropogenic and natural emissions
    Fu, Bo
    Jiang, Yongye
    Chen, Guolong
    Lu, Mengmeng
    Lai, Yuqin
    Suo, Xinhao
    Li, Bengang
    ENVIRONMENTAL RESEARCH LETTERS, 2024, 19 (06):
  • [44] Development of an anthropogenic atmospheric mercury emissions inventory in Thailand in 2018
    Pham Thi Bich Thao
    Pimonsree, Sittichai
    Suppoung, Kansak
    Bonnet, Sebastien
    Junpen, Agapol
    Garivait, Savitri
    ATMOSPHERIC POLLUTION RESEARCH, 2021, 12 (09)
  • [45] Anthropogenic Chloroform Emissions from China Drive Changes in Global Emissions
    An, Minde
    Western, Luke M.
    Hu, Jianxin
    Yao, Bo
    Muhle, Jens
    Ganesan, Anita L.
    Prinn, Ronald G.
    Krummel, Paul B.
    Hossaini, Ryan
    Fang, Xuekun
    O'Doherty, Simon
    Weiss, Ray F.
    Young, Dickon
    Rigby, Matthew
    ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2023, 57 (37) : 13925 - 13936
  • [46] Formation mechanism of heavy haze-fog associated with the interactions between different scales of atmospheric processes in China
    Deying Wang
    Jizhi Wang
    Yuanqin Yang
    Liangke Liu
    Junting Zhong
    Yaqiang Wang
    ATMOSPHERIC POLLUTION RESEARCH, 2021, 12 (06)
  • [47] Solar Brightening/Dimming over China's Mainland: Effects of Atmospheric Aerosols, Anthropogenic Emissions, and Meteorological Conditions
    Fang, Hejin
    Qin, Wenmin
    Wang, Lunche
    Zhang, Ming
    Yang, Xuefang
    REMOTE SENSING, 2021, 13 (01) : 1 - 18
  • [48] The Influence of Dynamics and Emissions Changes on China's Wintertime Haze
    Sherman, Peter
    Gao, Meng
    Song, Shaojie
    Ohiomoba, Patrick
    Archibald, Alex
    McElroy, Michael
    JOURNAL OF APPLIED METEOROLOGY AND CLIMATOLOGY, 2019, 58 (07) : 1603 - 1611
  • [49] Characteristics and Meteorological Factors of Severe Haze Pollution in China
    He, Chao
    Hong, Song
    Mu, Hang
    Tu, Peiyue
    Yang, Lu
    Ke, Biqin
    Huang, Jiayi
    ADVANCES IN METEOROLOGY, 2021, 2021
  • [50] Quantifying Concentrations and Emissions of Hexachlorobutadiene-A New Atmospheric Persistent Organic Pollutant in northern China
    Yang, Minmin
    Mao, Huiting
    Li, Hongli
    Yang, Fengchun
    Cao, Fangfang
    Wang, Yan
    ENVIRONMENTAL RESEARCH, 2023, 216