Efficient Photoelectrochemical Water Splitting by g-C3N4/TiO2 Nanotube Array Heterostructures

被引:140
|
作者
Liu, Changhai [1 ]
Wang, Fang [1 ]
Zhang, Jin [1 ]
Wang, Ke [1 ]
Qiu, Yangyang [1 ]
Liang, Qian [2 ]
Chen, Zhidong [2 ]
机构
[1] Changzhou Univ, Sch Mat Sci & Engn, Jiangsu Collaborat Innovat Ctr Photovolta Sci & E, Changzhou 213164, Jiangsu, Peoples R China
[2] Changzhou Univ, Sch Petrochem Engn, Changzhou 213164, Jiangsu, Peoples R China
基金
中国国家自然科学基金;
关键词
TiO2 nanotube arrays; Graphitic carbon nitride (g-C3N4); Heterojunction; Photoelectrochemical; Water splitting; TIO2 NANOWIRE ARRAYS; PHOTOCATALYTIC PERFORMANCE; HETEROJUNCTIONS; ANATASE; GROWTH; DEGRADATION; FABRICATION; COMPOSITES; CONVERSION; NANOSHEETS;
D O I
10.1007/s40820-018-0192-6
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Well-ordered TiO2 nanotube arrays (TNTAs) decorated with graphitic carbon nitride (g-C3N4) were fabricated by anodic oxidization and calcination process. First, TNTAs were prepared via the anodic oxidation of Ti foil in glycerol solution containing fluorinion and 20% deionized water. Subsequently, g-C3N4 film was hydrothermally grown on TNTAs via the hydrogen-bonded cyanuric acid melamine supramolecular complex. The results showed that g-C3N4 was successfully decorated on the TNTAs and the g-C3N4/TNTAs served as an efficient and stable photoanode for photoelectrochemical water splitting. The facile deposition method enables the fabrication of efficient and low-cost photoanodes for renewable energy applications. [GRAPHICS]
引用
收藏
页码:1 / 13
页数:13
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