Sewage Sludge-Derived Materials as Efficient Catalysts for the Selective Production of Vanillin from Isoeugenol

被引：19

作者：

Franco, Ana ^{[1
]}

Fernandes de Souza, Joao ^{[2
]}

Pinheiro do Nascimiento, Paula Fabiane ^{[2
]}

Mendes Pedroza, Marcelo ^{[2
]}

Santos de Carvalho, Luciene ^{[2
]}

Rodriguez-Castellon, Enrique ^{[3
]}

Luque, Rafael ^{[1
,4
]}

机构：

[1] Univ Cordoba, Dept Quim Organ, Campus Rabanales,Edificio Marie Curie C-3, Cordoba 14014, Spain

[2] Univ Fed Rio Grande do Norte, Dept Engn Quim, Inst Quim, Lab Tecnol Energet, BR-59078970 Natal, RN, Brazil

[3] Univ Malaga, Fac Ciencias, Dept Quim Inorgan Cristalog & Mineral, Campus Teatinos, E-29071 Malaga, Spain

[4] RUDN Univ, Peoples Friendship Univ Russia, 6 Miklukho Maklaya Str, Moscow 117198, Russia

来源：

ACS SUSTAINABLE CHEMISTRY & ENGINEERING | 2019年 / 7卷 / 08期

关键词：

Sewage sludge; Biochar; Oxidation; Vanillin; H2O2; OXIDATION; PYROLYSIS; EUGENOL; RISK; BIOTRANSFORMATION; CONVERSION; WATER;

D O I：

10.1021/acssuschemeng.8b05105

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Sewage sludge, a byproduct from wastewater treatment, is one of the most abundant residues in urban areas. Its high carbon and ash content make it an interesting waste to be potentially converted into novel materials via carbonization. In this work, we report the use of a sewage sludge material as the catalyst for the selective oxidation of isoeugenol to vanillin. High conversion (80%) and selectivity to vanillin (65%) were obtained after 1 h of reaction. Excellent material stability was observed after different catalytic reuses increasing the effectiveness of this material for catalytic applications.

引用

页码：7519 / 7526

页数：15

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