Ru Nanoparticles-Loaded Covalent Organic Framework for Solvent-Free One-Pot Tandem Reactions in Air

被引：76
|
作者：
Chen, Gong-Jun [1 ]
Li, Xiao-Bo [1 ]
Zhao, Chen-Chen [1 ]
Ma, Hui-Chao [1 ]
Kan, Jing-Lan [1 ]
Xin, Yu-Bin [1 ]
Chen, Cheng-Xia [2 ]
Dong, Yu-Bin [1 ]
机构：
[1] Shandong Normal Univ, Coll Chem Chem Engn & Mat Sci, Collaborat Innovat Ctr Functionalized Probes Chem, Key Lab Mol & Nano Probes,Minist Educ, Jinan 250014, Shandong, Peoples R China
[2] Sun Yat Sen Univ, Sch Chem & Chem Engn, MOE Lab Bioinorgan & Synthet Chem, Lehn Inst Funct Mat, Guangzhou 510275, Guangdong, Peoples R China
来源：
INORGANIC CHEMISTRY | 2018年 / 57卷 / 05期
关键词：
METAL NANOPARTICLES; CATALYTIC PERFORMANCE; ASYMMETRIC CATALYSIS; COUPLING REACTION; SUZUKI-MIYAURA; HYDROGENATION; OXIDATION; SIZE; GENERATION; CONVERSION;
D O I：
10.1021/acs.inorgchem.7b03077
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
Condensation of benzene-1,3,5-tricarbohydrazide with benzene-1,4-dicarboxaldehyde generated a new covalent organic framework, COF-ASB (1), in which the organic units are held together via hydrazone linkage to form porous frameworks. COF-ASB (1) is highly crystalline and displays good chemical and thermal stability and is permanently porous. In addition, 1 can be an ideal support to load Ru nanoparticles (Ru NPs) to generate Ru@COF-ASB (2). The obtained composite material is able to highly promote one-pot tandem synthesis of imine products from benzyl alcohols and corresponding amines under solvent-free conditions in air.
引用
收藏
页码：2678 / 2685
页数：8
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