Noble-Metal-Free Hybrid Membranes for Highly Efficient Hydrogen Evolution

被引：83

作者：

Wang, Xuyang ^{[1
]}

Gan, Xin ^{[1
,2
]}

Hu, Tao ^{[1
]}

Fujisawa, Kazunori ^{[3
]}

Lei, Yu ^{[4
,5
]}

Lin, Zhong ^{[3
]}

Xu, Ben ^{[1
]}

Huang, Zheng-Hong ^{[1
]}

Kang, Feiyu ^{[1
,2
]}

Terrones, Mauricio ^{[3
,4
,5
,6
,7
]}

Lv, Ruitao ^{[1
]}

机构：

[1] Tsinghua Univ, Key Lab Adv Mat MOE, Sch Mat Sci & Engn, Beijing 100084, Peoples R China

[2] Tsinghua Univ, Grad Sch Shenzhen, Shenzhen 518055, Peoples R China

[3] Penn State Univ, Dept Phys, 104 Davey Lab, University Pk, PA 16802 USA

[4] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA

[5] Penn State Univ, Ctr Dimens & Layered Mat 2, University Pk, PA 16802 USA

[6] Penn State Univ, Dept Chem, University Pk, PA 16802 USA

[7] Shinshu Univ, Inst Carbon Sci & Technol, Wakasato 4-17-1, Nagano 3808553, Japan

来源：

ADVANCED MATERIALS | 2017年 / 29卷 / 04期

基金：

美国国家科学基金会; 中国国家自然科学基金;

关键词：

ACTIVE EDGE SITES; ELECTROCHEMICAL H-2 EVOLUTION; MOS2 ULTRATHIN NANOSHEETS; REDUCED GRAPHENE OXIDE; CATALYTIC-ACTIVITY; WS2; NANOSHEETS; ELECTROCATALYSTS; IDENTIFICATION; PYROLYSIS; NANOWIRES;

D O I：

10.1002/adma.201603617

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Free-standing and flexible WS2/WO2.9/Chybrid membranes are synthesized and used as catalytic electrodes for electrochemical hydrogen evolution, exhibiting a high and stable catalytic activity. By virtue of the synergetic effect, a low onset overpotential of 20 mV and a Tafel slope of 36 mV dec(-1) are achieved.

引用

页数：8

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