Dynamics of polymer translocation into a circular nanocontainer through a nanopore

被引:18
|
作者
Zhang, Kehong [1 ,2 ]
Luo, Kaifu [1 ]
机构
[1] Univ Sci & Technol China, Dept Polymer Sci & Engn, CAS Key Lab Soft Matter Chem, Hefei 230026, Anhui Province, Peoples R China
[2] Anhui Agr Univ, Coll Light Text Engn & Art, Hefei 230036, Anhui Province, Peoples R China
来源
JOURNAL OF CHEMICAL PHYSICS | 2012年 / 136卷 / 18期
基金
中国国家自然科学基金;
关键词
DNA TRANSLOCATION; DRIVEN; MOLECULE; SIMULATION; TRANSPORT; MOTION; FORCE;
D O I
10.1063/1.4712618
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Using Langevin dynamics simulations, we investigate the dynamics of polymer translocation into a circular nanocontainer through a nanopore under a driving force F. We observe that the translocation probability initially increases and then saturates with increasing F, independent of phi, which is the average density of the whole chain in the nanocontainer. The translocation time distribution undergoes a transition from a Gaussian distribution to an asymmetric distribution with increasing phi. Moreover, we find a nonuniversal scaling exponent of the translocation time as chain length, depending on phi and F. These results are interpreted by the conformation of the translocated chain in the nanocontainer and the time of an individual segment passing through the pore during translocation. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4712618]
引用
收藏
页数:8
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