Long-range atmospheric transport of particulate Polycyclic Aromatic Hydrocarbons and the incursion of aerosols to the southeast Tibetan Plateau

被引:54
|
作者
Wang, Xiaoping [1 ,2 ]
Gong, Ping [1 ,2 ]
Sheng, Jiujiang [1 ]
Joswiak, Daniel R. [1 ]
Yao, Tandong [1 ,2 ]
机构
[1] Chinese Acad Sci, Key Lab Tibetan Environm Changes & Land Surface P, Inst Tibetan Plateau Res, Beijing 100101, Peoples R China
[2] CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing, Peoples R China
基金
中国国家自然科学基金;
关键词
Polycyclic Aromatic Hydrocarbons; Tibetan Plateau; Westerly winds; Himalayas; BLACK CARBON; ORGANOCHLORINE PESTICIDES; OPTICAL-PROPERTIES; SOURCE REGIONS; SOURCE APPORTIONMENT; SPATIAL-DISTRIBUTION; EMISSION INVENTORY; BROWN CLOUDS; PAHS; AIR;
D O I
10.1016/j.atmosenv.2015.04.050
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The long range atmospheric transport of Polycyclic Aromatic Hydrocarbons (PAHs) from heavily polluted regions to remote areas has been well-known. However, there are limited studies focussing on the Tibetan Plateau (TP). To assess the temporal transport patterns of PAHs and particulate matters (PMs), a ground-based observation program (2008-2011) was conducted in the southeast TP. Relatively high atmospheric concentrations of particulate-PAHs (0.2-5.0 ng m(-3), sum of 15 compounds) and Total suspended Particles (TSP, 4.1-46.7 mu g m(-3)) were observed. Concentrations of particulate-PAHsITSP exhibited seasonality with higher levels in the winter spring season and lower levels in summer. Using the potential source contribution function model, the source region of both particulate-PAHs and particles was attributed to the Indo-Gangetic Plain (IGP), suggesting the co-transport of particulate-PAHs and aerosols. The aerosol incursion, penetrating the Himalayas and reaching the TP was further captured by Moderate Resolution Imaging Spectroradiometer and Cloud-Aerosol Lidar Infrared Pathfinder Satellite Observations. (C) 2015 Elsevier Ltd. All rights reserved.
引用
收藏
页码:124 / 131
页数:8
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