How do aerosols above the residual layer affect the planetary boundary layer height?

被引:39
|
作者
Ma, Yongjing [1 ]
Xin, Jinyuan [1 ,2 ]
Wang, Zifa [1 ]
Tian, Yongli [3 ]
Wu, Lin [1 ]
Tang, Guiqian [1 ]
Zhang, Wenyu [4 ]
de Arellano, Jordi Vila-Guerau [5 ]
Zhao, Dandan [1 ,2 ]
Jia, Danjie [1 ,2 ]
Ren, Yuanzhe [3 ]
Gao, Zhongming [6 ]
Shen, Pengke [7 ]
Ye, Jianhuai [8 ]
Martin, Scot T. [8 ]
机构
[1] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[3] Inner Mongolia Autonomous Reg Environm Monitoring, Hohhot 010090, Peoples R China
[4] Zhengzhou Univ, Sch Geosci & Technol, Zhengzhou 450001, Peoples R China
[5] Wageningen Univ, Meteorol & Air Qual, Wageningen, Netherlands
[6] Sun Yat Sen Univ, Sch Atmospher Sci, Zhuhai 519000, Peoples R China
[7] Peking Univ, Coll Urban & Environm Sci, Key Lab Earth Surface Proc, Minist Educ, Beijing 100871, Peoples R China
[8] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA
基金
中国国家自然科学基金;
关键词
Large-eddy simulation; Planetary boundary layer; Virtual dome effect; Aloft umbrella effect; Dome effective height; BLACK CARBON; POLLUTION; CHINA; HAZE; ABSORPTION;
D O I
10.1016/j.scitotenv.2021.151953
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
We revealed that the absorption aerosol lying below or above the morning residual layer (MRL) promotes (stove effect, heating the MRL layer) or strongly inhibits (dome effect, heating the temperature inversion layer) the development of planetary boundary layer (PBL) after sunrise, while scattering aerosol exhibits similar suppression (surface or aloft umbrella effect) on the PBL regardless of its vertical location. However, the role of different type of aerosols (i.e., strong absorption aerosol and purely scattering aerosol) present from MRL to upper atmosphere remains lacking and therefore, needs to be further explored. Utilizing a large-eddy simulation model constrained by the in-situ observations in urban Beijing, we observed that the dome inhibition of absorption aerosols on PBL development becomes weaker as elevating the aerosol layer, and the effect (virtual dome effect) remains no change beyond a certain height, which is defined as the dome effective height z. This height z is highly related to the surface sensible heat flux. By comparison, the altitude of light-scattering aerosols relative to the MRL was less important. The scattering aerosols exhibit similar inhibition from MRL to upper atmosphere (aloft umbrella effect), but to a weaker extent than the virtual dome effect. The virtual dome effect and aloft umbrella effect play a leading role during some extremely polluted scenarios with deep aerosol layer, such as sandstorms and volcanic eruptions. Aerosol dome, virtual dome, and aloft umbrella effects, together with aerosol stove and surface umbrella effects, further advance the understanding on aerosol-PBL interactions, which is, more broadly, applied to interpret the impact of aerosol on PBL over other ecosystems as well as exoplanet atmospheres.
引用
收藏
页数:9
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