Biomass-derived 3D evaporator with antifouling and salt-rejecting toward solar-enabled steam generation, desalination, and electricity generation

被引:23
|
作者
Ma, Wenjing [1 ]
Cao, Wenxuan [1 ]
Cui, Min [1 ]
Lu, Haifeng [2 ]
Xiong, Ranhua [1 ]
Huang, Chaobo [1 ]
机构
[1] Nanjing Forestry Univ, Jiangsu Coinnovat Ctr Efficient Proc & Utilizat Fo, Joint Lab Adv Biomed Mat NFU UGent, Nanjing 210037, Peoples R China
[2] Zhejiang Normal Univ, Inst Sci & Applicat Mol Ferroelect, Key Lab, Minist Educ Adv Catalysis Mat, Jinhua 321004, Peoples R China
基金
中国国家自然科学基金;
关键词
Solar evaporation; Water purification; Electricity generation; Natural sorghum stalks pitch; Zwitterionic hydrogels; Biomass-derived 3D evaporator; HIGHLY EFFICIENT; WATER DESALINATION; ATTAPULGITE; MEMBRANE; FOAMS;
D O I
10.1016/j.cej.2023.147404
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Solar-driven interfacial evaporation is currently considered as one of the most effective and sustainable strategies to address water scarcity and energy shortages issues. Whereas, challenges in developing durable, eco-friendly, and low-cost solar evaporators from readily available materials still exist. Herein, we have reported a facile strategy to construct a robust natural sorghum stalk pith solar evaporator. With advantageous features of gradient honeycomb structure and hydrophilic polymer chains, the constructed evaporator exhibits broadband light absorption, efficient light to heat conversion, fast water transport, and multi-channel release of steam performances, leading to an ultrahigh evaporation rate of 3.79 kg m(-2)h(-1) under one sun irradiation and outstanding salt-resistant ability at a high evaporation rate of 2.6 kg<middle dot>m(-2)<middle dot>h(-1) in a highly concentrated brine (20 wt% NaCl), accompanied with anti-oil-fouling performances, as well as high oil removal efficiency (>99.8 %) for oil-in-water emulsion, outperforming most previously reported solar evaporators. Additionally, solar irradiation can further promote the directional water flow, contributing to a high photovoltage of 68 mV under one sun illumination. This paves the way for designing durable biomass-based steam generators, not only scaling up sustainable clean water production, sewage depuration and desalination, but also discovering promising application in the field of electricity generation.
引用
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页数:10
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