CH4;
remote sensing;
detection probability;
sensitivity;
aggregation;
point source;
NATURAL-GAS;
D O I:
10.1021/acs.est.3c00229
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
Aerial LiDAR measurements at 7474 oil and gas productionfacilitiesin the Permian Basin yield a measured methane emission rate distributionextending to the detection sensitivity of the method, 2 kg/h at 90%probability of detection (POD). Emissions are found at 38.3% of facilitiesscanned, a significantly higher proportion than reported in lower-sensitivitycampaigns. LiDAR measurements are analyzed in combination with measurementsof the heavy tail portion of the distribution (>600 kg/h) obtainedfrom an airborne solar infrared imaging spectrometry campaign by CarbonMapper (CM). A joint distribution is found by fitting the alignedLiDAR and CM data. By comparing the aerial samples to the joint distribution,the practical detection sensitivity of the CM 2019 campaign is foundto be 280 kg/h [256, 309] (95% confidence) at 50% POD for facility-sizedemission sources. With respect to the joint model distribution andits confidence interval, the LiDAR campaign is found to have measured103.6% [93.5, 114.2%] of the total emission rate predicted by themodel for equipment-sized emission sources (& SIM;2 m diameter)with emission rates above 3 kg/h, whereas the CM 2019 campaign isfound to have measured 39.7% [34.6, 45.1%] of the same quantity forfacility-sized sources (150 m diameter) above 10 kg/h. The analysisis repeated with data from CM 2020-21 campaigns with similarresults. The combined distributions represent a more comprehensiveview of the emission rate distribution in the survey area, revealingthe significance of previously underreported emission sources at ratesbelow the detection sensitivity of some emissions monitoring campaigns. New methane emission measurements inthe Permian Basin extendthe distribution of source emission rates beyond the sensitivity limitsof previous studies by 2 orders of magnitude.
机构:
Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO 80305 USA
Calif Air Resources Board, Sacramento, CA 95814 USAUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
Cui, Yu Yan
Henze, Daven K.
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机构:
Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USAUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
Henze, Daven K.
Brioude, Jerome
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机构:
Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO 80305 USA
Univ La Reunion, Meteo France, CNRS, UMR8105,Lab Atmosphere & Cyclones, La Reunion, FranceUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
Brioude, Jerome
Angevine, Wayne M.
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机构:
Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO 80305 USAUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
Angevine, Wayne M.
Liu, Zhen
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h-index: 0
机构:
Calif Air Resources Board, Sacramento, CA 95814 USA
Ramboll Environ US Corp, Novato, CA USAUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
Liu, Zhen
Bousserez, Nicolas
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Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USAUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
Bousserez, Nicolas
Guerrette, Jonathan
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机构:
Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO 80305 USAUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
Guerrette, Jonathan
McKeen, Stuart A.
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机构:
Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO 80305 USAUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
McKeen, Stuart A.
Peischl, Jeff
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机构:
Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO 80305 USAUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
Peischl, Jeff
Yuan, Bin
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机构:
Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO 80305 USAUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
Yuan, Bin
Ryerson, Thomas
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NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO 80305 USAUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
Ryerson, Thomas
Frost, Gregory
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NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO 80305 USAUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
Frost, Gregory
Trainer, Michael
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机构:
NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO 80305 USAUniv Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA