Asymmetric solar evaporator with salt-resistance capability for freshwater and energy generation

被引:18
|
作者
Wang, Lifeng [1 ]
Ma, Yuxi [1 ]
Yang, Guoliang [1 ]
Li, Xuefei [2 ]
Liu, Dan [1 ]
Qin, Si [1 ]
Lei, Weiwei [1 ]
机构
[1] Deakin Univ, Inst Frontier Mat, Waurn Ponds Campus, Locked Bag 20000, Geelong, Vic 3220, Australia
[2] Jilin Normal Univ, Key Lab Funct Mat Phys & Chem, Minist Educ, Changchun 130000, Peoples R China
基金
澳大利亚研究理事会;
关键词
Janus solar evaporator; Clean water generation; Salt-resistance; Energy generation; STEAM-GENERATION; EFFICIENT;
D O I
10.1016/j.cej.2023.144761
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Solar-driven steam generation is a promising solution for addressing the pressing challenges of freshwater and energy scarcity, but the accumulation of salt on the evaporator surface hinders performance by reducing sunlight absorption and blocking water transport. To overcome this limitation, we developed an innovative Janus solar evaporator with asymmetric surface wettability that simultaneously generates energy and clean water. The solar evaporator-based niobium nitride (Nb4N5) nanosheets with broadband absorption and high light-to-thermal conversion capability displayed an excellent high evaporation rate of 2.30 kg m-2 h-1 under 1 kW m-2 irradiation, which was 4.8-fold higher than that of melamine foam evaporator. Notably, the Janus evaporators displayed an excellent evaporation rate of up to 2.10 kg m-2 h-1 in 20wt.% NaCl solution. Furthermore, during steam generation, the hybrid evaporator with a thermo-electricity module produced an open-circuit voltage of 135 mV and a short-circuit current of 14.6 mA under two sun irradiation. Our findings demonstrated that the Janus evaporator with salt-resistance property has significant potential for simultaneous steam and electricity production, offering a promising solution to simultaneously address the water and energy crisis.
引用
收藏
页数:7
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