Pt-Zn Bimetallic Nanoclusters Encapsulated in SAPO-11 Molecular Sieve with Excellent Catalytic Performance for Levulinic Acid Hydrogenation

被引：2
|
作者：
Huang, Yanli [1 ]
Wang, Yanyun [1 ]
Zuo, Changjiang [1 ]
Sheng, Xiaoli [1 ]
Huang, Yuzhong [2 ]
Zhang, Yiwei [1 ]
Zhou, Yuming [1 ]
机构：
[1] Southeast Univ, Sch Chem & Chem Engn, Jiangsu Optoelect Funct Mat & Engn Lab, Nanjing 211189, Peoples R China
[2] ZYfire Hose Co Ltd, Taizhou 225599, Jiangsu, Peoples R China
来源：
CATALYSIS LETTERS | 2023年 / 153卷 / 09期
基金：
中国国家自然科学基金;
关键词：
Levulinic acid; Hydrogenation; Zeolite; Encapsulation; Platinum; SILICALITE-1; ZEOLITE; NANOPARTICLES; METAL; ZSM-5; PT/SAPO-11; DESIGN;
D O I：
10.1007/s10562-022-04147-4
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Well-dispersed Pt-Zn nanoclusters encapsulated in the mesopores of SAPO-11 were prepared by a one-pot synthesis method using dipropylamine to anchor metal nanoclusters to the support. The phenomenon of metal leaching or agglomeration can be effectively avoided. It exhibits high stability after 36 h of reaction time, with a GVL yield above 80%. [GRAPHICAL ABSTRACT]
引用
收藏
页码：2651 / 2664
页数：14
相关论文
共 41 条
  • [31] Synthesis of ZSM-22/SAPO-11 composite molecular sieve-based catalysts with small crystallites and superior n-alkane hydroisomerization performance
    Wang, Xue-Man
    Wen, Cheng-Long
    Fan, Yu
    PETROLEUM SCIENCE, 2023, 20 (04) : 2585 - 2595
  • [32] Synthesis of ZSM-22/SAPO-11 composite molecular sieve-based catalysts with small crystallites and superior n-alkane hydroisomerization performance
    XueMan Wang
    ChengLong Wen
    Yu Fan
    Petroleum Science, 2023, 20 (04) : 2585 - 2595
  • [33] Highly mesoporous SAPO-11 molecular sieves with tunable acidity: facile synthesis, formation mechanism and catalytic performance in hydroisomerization of n-dodecane
    Tao, Shuo
    Li, Xiaolei
    Lv, Guang
    Wang, Congxin
    Xu, Renshun
    Ma, Huaijun
    Tian, Zhijian
    CATALYSIS SCIENCE & TECHNOLOGY, 2017, 7 (23) : 5775 - 5784
  • [34] Small-crystal and hierarchical SAPO-11 molecular sieve synthesized via three-stage crystallization method and hydroisomerization performance of corresponding NiWS supported catalyst
    Dai, Xiaojun
    Cheng, Yan
    Wei, Qiang
    Si, Meng
    Zhou, Yasong
    FUEL, 2022, 324
  • [35] Small-crystal and hierarchical SAPO-11 molecular sieve synthesized via three-stage crystallization method and hydroisomerization performance of corresponding NiWS supported catalyst
    Dai, Xiaojun
    Cheng, Yan
    Wei, Qiang
    Si, Meng
    Zhou, Yasong
    Fuel, 2022, 324
  • [36] In-situ Synthesis of Gallium-Containing SAPO-11 Molecular Sieves and Superior Catalytic Performance of Their NiWS Supported Catalysts for Hydroisomerization of n-Hexadecane
    Dai, Xiaojun
    Li, Ling
    Cheng, Yan
    Yu, Wanjin
    Liu, Wucan
    Yang, Han
    Si, Meng
    Wei, Qiang
    Zhou, Yasong
    EUROPEAN JOURNAL OF INORGANIC CHEMISTRY, 2023, 26 (02)
  • [37] Novel synthesis strategy of SAPO-11 molecular sieve with superior performance for hydroisomerization of long-chain n-alkanes: Supergravity-cyclone assisted hydrothermal crystallization method
    Dai, Xiaojun
    Cheng, Yan
    Liu, Tingting
    Wei, Qiang
    Zhou, Yasong
    CHEMICAL ENGINEERING JOURNAL, 2023, 472
  • [38] Synthesis of nano-sized small-crystal and hierarchical SAPO-11 molecular sieves and superior catalytic performance of their NiWS-supported catalysts in hydroisomerization of n-hexadecane
    Dai, Xiaojun
    Cheng, Yan
    Wei, Qiang
    Si, Meng
    Zhang, Pengfei
    Zhou, Yasong
    MICROPOROUS AND MESOPOROUS MATERIALS, 2022, 343
  • [39] Template/Al2O3 Ratio in Reaction Gels as a Tool to Control the Crystal Morphology, Crystal Dispersion, and Catalytic Performance in Hydroisomerization of n-Hexadecane over SAPO-11 Molecular Sieves
    Serebrennikov, D. V.
    Zabirov, A. R.
    Kuvatova, R. Z.
    Bagdanova, D. O.
    Malunov, A. I.
    Dement'ev, K. I.
    Agliullin, M. R.
    PETROLEUM CHEMISTRY, 2024, 64 (11) : 1276 - 1285
  • [40] Design of Pt/SAPO-11 bifunctional catalyst with superior metal-acid balance constructed via a novel one-step pre-loading strategy for enhancing n-dodecane hydroisomerization performance
    Du, Yanyan
    Yao, Heliang
    Hu, Wenjing
    Tan, Yangchun
    Xu, Yanhui
    Fu, Wenjia
    Yuan, Long
    Li, Jiusheng
    CATALYSIS SCIENCE & TECHNOLOGY, 2020, 10 (17) : 5953 - 5963
12345