Design and Synthesis of Bistetrazole-Based Energetic Salts Bearing the Nitrogen-Rich Fused Ring

被引：5

作者：

Cui, Wen-Hao ^{[1
]}

Liu, Qi ^{[1
]}

Ye, Zhiwen ^{[1
]}

He, Ying ^{[1
]}

机构：

[1] Nanjing Univ Sci & Technol, Sch Chem & Chem Engn, Nanjing 210094, Jiangsu, Peoples R China

来源：

ORGANIC LETTERS | 2023年 / 25卷 / 30期

关键词：

DIMROTH REARRANGEMENT; TETRAZOLES; COMPLEX;

D O I：

10.1021/acs.orglett.3c02131

中图分类号：

O62 [有机化学];

学科分类号：

070303 ; 081704 ;

摘要：

A series of bistetrazole-based energetic salts bearinga nitrogen-richfused ring were designed and synthesized. Among them, compounds 4-10 showed good detonation propertiesand excellent thermostability. By treating nitrogen-rich fused ring 3 with concentrated hydrochloric acid, a new type of Dimrothrearrangement was observed that afforded compound 12 efficiently.This new transformation herein constitutes a valuable addition tothe Dimroth rearrangement.

引用

页码：5661 / 5665

页数：5

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