Design and Synthesis of Bistetrazole-Based Energetic Salts Bearing the Nitrogen-Rich Fused Ring

被引：5
|
作者：
Cui, Wen-Hao [1 ]
Liu, Qi [1 ]
Ye, Zhiwen [1 ]
He, Ying [1 ]
机构：
[1] Nanjing Univ Sci & Technol, Sch Chem & Chem Engn, Nanjing 210094, Jiangsu, Peoples R China
来源：
ORGANIC LETTERS | 2023年 / 25卷 / 30期
关键词：
DIMROTH REARRANGEMENT; TETRAZOLES; COMPLEX;
D O I：
10.1021/acs.orglett.3c02131
中图分类号：
O62 [有机化学];
学科分类号：
070303 ; 081704 ;
摘要：
A series of bistetrazole-based energetic salts bearinga nitrogen-richfused ring were designed and synthesized. Among them, compounds 4-10 showed good detonation propertiesand excellent thermostability. By treating nitrogen-rich fused ring 3 with concentrated hydrochloric acid, a new type of Dimrothrearrangement was observed that afforded compound 12 efficiently.This new transformation herein constitutes a valuable addition tothe Dimroth rearrangement.
引用
收藏
页码：5661 / 5665
页数：5
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