Boron monosulfide as an electrocatalyst for the oxygen evolution reaction

被引：15

作者：

Li, Linghui ^{[1
]}

Hagiwara, Satoshi ^{[2
]}

Jiang, Cheng ^{[3
]}

Kusaka, Haruki ^{[1
]}

Watanabe, Norinobu ^{[1
]}

Fujita, Takeshi ^{[4
]}

Kuroda, Fumiaki ^{[2
]}

Yamamoto, Akiyasu ^{[5
]}

Miyakawa, Masashi ^{[6
]}

Taniguchi, Takashi ^{[6
]}

Hosono, Hideo ^{[6
,7
]}

Otani, Minoru ^{[2
]}

Kondo, Takahiro ^{[8
,9
,10
,11
]}

机构：

[1] Univ Tsukuba, Grad Sch Pure & Appl Sci, Tsukuba 3058573, Japan

[2] Univ Tsukuba, Ctr Computat Sci, Tsukuba 3058571, Japan

[3] Rhein Westfal TH Aachen, Inst Tech & Macromol Chem, D-52074 Aachen, Germany

[4] Kochi Univ Technol, Sch Engn Sci, Kochi 7828502, Japan

[5] Tokyo Univ Agr & Technol, Tokyo 1838538, Japan

[6] Natl Inst Mat Sci, Res Ctr Mat Nanoarchitecton, Tsukuba 3050044, Japan

[7] Tokyo Inst Technol, MDX Res Ctr Element Strategy, Yokohama 2268503, Japan

[8] Univ Tsukuba, Dept Mat Sci, Tsukuba 3058573, Japan

[9] Univ Tsukuba, Inst Pure & Appl Sci, Tsukuba Res Ctr Energy Mat Sci, Tsukuba 3058573, Japan

[10] Univ Tsukuba, R&D Ctr Zero Emiss Funct Mat CO2, Tsukuba 3058573, Japan

[11] Tohoku Univ, Adv Inst Mat Res, Sendai 9808577, Japan

来源：

CHEMICAL ENGINEERING JOURNAL | 2023年 / 471卷

关键词：

Boron monosulfide; Electrocatalyst; Oxygen evolution reaction; Alkaline medium; Graphene; Renewable energy device; REDUCTION;

D O I：

10.1016/j.cej.2023.144489

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

The current energy crisis and environmental problems associated with the use of fossil fuels necessitate a transition to clean and sustainable energy carriers like hydrogen produced by electrocatalytic water splitting. Hence, the development of robust, low-cost, and high-performance oxygen evolution reaction (OER) electrocatalysts has attracted considerable attention. Herein, an OER electrocatalyst for use in alkaline media is prepared by hybridising rhombohedral boron monosulfide with graphene to provide electronic conductivity. The catalytic activity of the electrocatalyst (overpotential of 250 mV at 10 mA cm-2) is higher than those of most previously reported counterparts. Our results pave the way for the design of electrocatalysts composed of abundant elements with a wide range of applications in renewable energy devices.

引用

页数：9

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