High-energy molecular-frame photoelectron angular distributions: a molecular bond-length ruler

被引：7

作者：

Vela-Perez, I. ^{[1
]}

Ota, F. ^{[2
]}

Mhamdi, A. ^{[3
,4
]}

Tamura, Y. ^{[2
]}

Rist, J. ^{[1
]}

Melzer, N. ^{[1
]}

Uerken, S. ^{[1
]}

Nalin, G. ^{[1
]}

Anders, N. ^{[1
]}

You, D. ^{[5
]}

Kircher, M. ^{[1
]}

Janke, C. ^{[1
]}

Waitz, M. ^{[1
]}

Trinter, F. ^{[6
,7
]}

Guillemin, R. ^{[8
]}

Piancastelli, M. N. ^{[8
]}

Simon, M. ^{[8
]}

Davis, V. T. ^{[9
]}

Williams, J. B. ^{[9
]}

Doerner, R. ^{[1
]}

Hatada, K. ^{[2
]}

Yamazaki, K. ^{[10
]}

Fehre, K. ^{[1
]}

Demekhin, Ph. V. ^{[3
,4
]}

Ueda, K. ^{[5
,11
]}

Schoeffler, M. S. ^{[1
]}

Jahnke, T. ^{[12
]}

机构：

[1] Goethe Univ, Inst Kernphys, Max von Laue Str 1, D-60438 Frankfurt, Germany

[2] Univ Toyama, Dept Phys, Gofuku 3190, Toyama 9308555, Japan

[3] Univ Kassel, Inst Phys, Heinrich Plett Str 40, D-34132 Kassel, Germany

[4] Univ Kassel, CINSaT, Heinrich Plett Str 40, D-34132 Kassel, Germany

[5] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan

[6] Deutsch Elektronen Synchrotron DESY, Notkestr 85, D-22607 Hamburg, Germany

[7] Max Planck Gesell, Fritz Haber Inst, Mol Phys, Faradayweg 4-6, D-14195 Berlin, Germany

[8] Sorbonne Univ, CNRS, LCPMR, F-75005 Paris, France

[9] Univ Nevada, Dept Phys, Reno, NV 89557 USA

[10] RIKEN, RIKEN Ctr Adv Photon, 2-1 Hirosawa, Wako, Saitama 3510198, Japan

[11] Tohoku Univ, Dept Chem, 6-3 Aramaki Aza Aoba,Aoba Ku, Sendai, Miyagi 9808578, Japan

[12] European XFEL, Holzkoppel 4, D-22869 Schenefeld, Germany

来源：

PHYSICAL CHEMISTRY CHEMICAL PHYSICS | 2023年 / 25卷 / 19期

关键词：

INFORMATION;

D O I：

10.1039/d2cp05942h

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We present a study on molecular-frame photoelectron angular distributions (MFPADs) of small molecules using circularly polarized synchrotron light. We find that the main forward-scattering peaks of the MFPADs are slightly tilted with respect to the molecular axis. This tilt angle is directly connected to the molecular bond length by a simple, universal formula. We apply the derived formula to several examples of MFPADs of C 1s and O 1s photoelectrons of CO, which have been measured experimentally or obtained by means of ab initio modeling. In addition, we discuss the influence of the back-scattering contribution that is superimposed over the analyzed forward-scattering peak in the case of homo-nuclear diatomic molecules such as N-2.

引用

页码：13784 / 13791

页数：8

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