Metal chalcogens;
Metallic sulfide and selenides;
Electrochemical water splitting;
Oxygen evolution reaction (OER);
OXYGEN EVOLUTION REACTION;
ELECTROCATALYSTS;
D O I:
10.1007/s43207-024-00372-2
中图分类号:
TQ174 [陶瓷工业];
TB3 [工程材料学];
学科分类号:
0805 ;
080502 ;
摘要:
To drive clean and sustainable fuel production via water electrolysis, development of high-performing, cost-effective electrocatalysts rich in earth elements without relying on precious metals or costly materials is crucial. In this study, strontium selenide (SrSe), copper sulfide (CuS), and composite SrSe@CuS via a traditional coprecipitate method under alkaline conditions are synthesized. Characterization techniques including X-ray diffraction, Transmission electron microscopy, Field emission scanning electron microscopy, and Brunauer-Emmett-Teller surface area analysis are employed to analyze the structure, morphology, and surface characteristics. The larger surface area of 123 m2 g-1 and lower crystalline size (46.43 nm) of SrSe@CuS nanosheets show more active sites for oxygen evolution reaction. The oxygen evolution activity displayed overpotentials of 290 mV, a lower tafel slope of 67 mV dec-1, and Lower charge transfer resistance (RCT) values of SrSe@CuS nanosheets (1.82 omega) surpassing the individual SrSe and CuS nanosheets. Notably, the SrSe@CuS nanosheets exhibited remarkable stability, maintaining an oxygen evolution reaction (OER) activity of 10 mA cm-2 for over 50 h and sustaining a negligible loss in performance even after 50,000 cycles of repetitive cyclivoltammetry scans. These findings highlight their potential applicability in energy conversion and storage systems.
机构:
Northwestern Polytech Univ, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Shaanxi Engn Lab Graphene New Carbon Mat & Applic, State Key Lab Solidificat Proc,Sch Mat Sci & Engn, Xian 710072, Shaanxi, Peoples R ChinaNorthwestern Polytech Univ, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Shaanxi Engn Lab Graphene New Carbon Mat & Applic, State Key Lab Solidificat Proc,Sch Mat Sci & Engn, Xian 710072, Shaanxi, Peoples R China
Zhao, Tingkai
Peng, Xiarong
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h-index: 0
机构:
Northwestern Polytech Univ, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Shaanxi Engn Lab Graphene New Carbon Mat & Applic, State Key Lab Solidificat Proc,Sch Mat Sci & Engn, Xian 710072, Shaanxi, Peoples R ChinaNorthwestern Polytech Univ, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Shaanxi Engn Lab Graphene New Carbon Mat & Applic, State Key Lab Solidificat Proc,Sch Mat Sci & Engn, Xian 710072, Shaanxi, Peoples R China
Peng, Xiarong
Zhao, Xin
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h-index: 0
机构:
NPU, Queen Mary Univ London Engn Sch, Xian 710072, Shaanxi, Peoples R ChinaNorthwestern Polytech Univ, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Shaanxi Engn Lab Graphene New Carbon Mat & Applic, State Key Lab Solidificat Proc,Sch Mat Sci & Engn, Xian 710072, Shaanxi, Peoples R China
Zhao, Xin
Hu, Jingtian
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h-index: 0
机构:
Northwestern Polytech Univ, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Shaanxi Engn Lab Graphene New Carbon Mat & Applic, State Key Lab Solidificat Proc,Sch Mat Sci & Engn, Xian 710072, Shaanxi, Peoples R ChinaNorthwestern Polytech Univ, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Shaanxi Engn Lab Graphene New Carbon Mat & Applic, State Key Lab Solidificat Proc,Sch Mat Sci & Engn, Xian 710072, Shaanxi, Peoples R China
Hu, Jingtian
Yang, Wenbo
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h-index: 0
机构:
Northwestern Polytech Univ, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Shaanxi Engn Lab Graphene New Carbon Mat & Applic, State Key Lab Solidificat Proc,Sch Mat Sci & Engn, Xian 710072, Shaanxi, Peoples R ChinaNorthwestern Polytech Univ, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Shaanxi Engn Lab Graphene New Carbon Mat & Applic, State Key Lab Solidificat Proc,Sch Mat Sci & Engn, Xian 710072, Shaanxi, Peoples R China
Yang, Wenbo
Li, Tiehu
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h-index: 0
机构:
Northwestern Polytech Univ, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Shaanxi Engn Lab Graphene New Carbon Mat & Applic, State Key Lab Solidificat Proc,Sch Mat Sci & Engn, Xian 710072, Shaanxi, Peoples R ChinaNorthwestern Polytech Univ, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Shaanxi Engn Lab Graphene New Carbon Mat & Applic, State Key Lab Solidificat Proc,Sch Mat Sci & Engn, Xian 710072, Shaanxi, Peoples R China
Li, Tiehu
Ahmad, Ishaq
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h-index: 0
机构:
Natl Ctr Phys, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Expt Phys Dept, Islamabad 44000, PakistanNorthwestern Polytech Univ, NPU NCP Joint Int Res Ctr Adv Nanomat & Defects E, Shaanxi Engn Lab Graphene New Carbon Mat & Applic, State Key Lab Solidificat Proc,Sch Mat Sci & Engn, Xian 710072, Shaanxi, Peoples R China
机构:
Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R China
Univ Sci & Technol China, Hefei 230026, Anhui, Peoples R ChinaChinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R China
Liu, Hanmeng
Wang, Yilin
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h-index: 0
机构:
Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R China
Univ Chinese Acad Sci, Beijing 100049, Peoples R ChinaChinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R China
Wang, Yilin
Li, Zhen
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h-index: 0
机构:
Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R China
Univ Chinese Acad Sci, Beijing 100049, Peoples R ChinaChinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R China
Li, Zhen
Yao, Zhixia
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h-index: 0
机构:
Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R China
Univ Chinese Acad Sci, Beijing 100049, Peoples R ChinaChinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R China
Yao, Zhixia
Lin, Jing
论文数: 0引用数: 0
h-index: 0
机构:
Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R China
Jilin Normal Univ, Coll Chem, Jilin 136000, Jilin, Peoples R ChinaChinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R China
Lin, Jing
Sun, Yujing
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h-index: 0
机构:
Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R ChinaChinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R China
Sun, Yujing
Li, Zhuang
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h-index: 0
机构:
Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R ChinaChinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Jilin, Peoples R China
机构:
College of Chemistry and Chemical Engineering, Anyang Normal UniversityCollege of Chemistry and Chemical Engineering, Anyang Normal University
Junhong Zhao
Jinping Wu
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h-index: 0
机构:
College of Chemistry and Chemical Engineering, Anyang Normal UniversityCollege of Chemistry and Chemical Engineering, Anyang Normal University
Jinping Wu
Bing Li
论文数: 0引用数: 0
h-index: 0
机构:
College of Chemistry and Chemical Engineering, Yangzhou UniversityCollege of Chemistry and Chemical Engineering, Anyang Normal University
Bing Li
Weimin Du
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h-index: 0
机构:
College of Chemistry and Chemical Engineering, Anyang Normal UniversityCollege of Chemistry and Chemical Engineering, Anyang Normal University
Weimin Du
Qingli Huang
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h-index: 0
机构:
College of Chemistry and Chemical Engineering, Anyang Normal UniversityCollege of Chemistry and Chemical Engineering, Anyang Normal University
Qingli Huang
Mingbo Zheng
论文数: 0引用数: 0
h-index: 0
机构:
College of Chemistry and Chemical Engineering, Yangzhou UniversityCollege of Chemistry and Chemical Engineering, Anyang Normal University
Mingbo Zheng
Huaiguo Xue
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h-index: 0
机构:
College of Chemistry and Chemical Engineering, Yangzhou UniversityCollege of Chemistry and Chemical Engineering, Anyang Normal University
Huaiguo Xue
Huan Pang
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h-index: 0
机构:
College of Chemistry and Chemical Engineering, Anyang Normal University
College of Chemistry and Chemical Engineering, Yangzhou UniversityCollege of Chemistry and Chemical Engineering, Anyang Normal University
机构:
Univ Guilan, Fac Sci, Dept Phys, POB 41335, Rasht, Iran
Payame Noor Univ, Dept Phys, POB 19395-3697, Tehran, IranUniv Guilan, Fac Sci, Dept Phys, POB 41335, Rasht, Iran
Askari, Mohammad Bagher
Salarizadeh, Parisa
论文数: 0引用数: 0
h-index: 0
机构:
Vali E Asr Univ Rafsanjan, High Temp Fuel Cell Res Dept, Rafsanjan 1599637111, IranUniv Guilan, Fac Sci, Dept Phys, POB 41335, Rasht, Iran
Salarizadeh, Parisa
Seifi, Majid
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h-index: 0
机构:
Univ Guilan, Fac Sci, Dept Phys, POB 41335, Rasht, IranUniv Guilan, Fac Sci, Dept Phys, POB 41335, Rasht, Iran
Seifi, Majid
Rozati, Seyed Mohammad
论文数: 0引用数: 0
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机构:
Univ Guilan, Fac Sci, Dept Phys, POB 41335, Rasht, IranUniv Guilan, Fac Sci, Dept Phys, POB 41335, Rasht, Iran