Distributions and potential sources of polychlorinated biphenyls and polycyclic aromatic hydrocarbons in the glacimarine sediments of Arctic Svalbard

被引:7
|
作者
Lee, Juhee [1 ]
Kim, Youngnam [1 ]
Cha, Jihyun [1 ]
Kim, Dahae [2 ,3 ]
Jang, Kwangchul [2 ]
Kim, Jung-Hyun [2 ]
Nam, Seung-Il [2 ]
Hong, Seongjin [1 ]
机构
[1] Chungnam Natl Univ, Dept Marine Environm Sci, Daejeon 34134, South Korea
[2] Korea Polar Res Inst, Div Glacial Environm Res, Incheon 21990, South Korea
[3] Hanyang Univ ERICA Campus, Dept Marine Sci & Convergence Technol, Ansan 15588, South Korea
基金
新加坡国家研究基金会;
关键词
Persistent toxic substances; Arctic Svalbard; Mining activity; Alkyl-PAHs; Sediment; PERSISTENT ORGANIC POLLUTANTS; SOURCE IDENTIFICATION; SPATIAL-DISTRIBUTION; ENVIRONMENTAL FATE; COASTAL SEDIMENTS; MARINE-SEDIMENTS; PAH SOURCE; PCBS; SOILS; LAKE;
D O I
10.1016/j.marpolbul.2023.114740
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Distribution and sources of polychlorinated biphenyls (PCBs) and polycyclic aromatic hydrocarbons (PAHs) in the glacimarine sediments (35 sites) of Svalbard were investigated. PCBs (32 congeners), traditional PAHs (15 homologs), emerging PAHs (11 homologs), and alkylated PAHs (16 homologs) were widely distributed in the Svalbard sediments (ranges: below method detection limit to 20, 21 to 3600, 1.0 to 1400, and 31 to 15,000 ng g-1 dry weight, respectively). Compositional analysis indicated that PCBs mainly originated from combustion sources, with PAHs being strongly influenced by local sources. Positive matrix factorization analysis showed that PAHs were associated with vehicle and petroleum combustion, coal, and coal combustion. Coal-derived PAHs contributed significantly to the sediments of Van Mijenfjorden. Remnants of coal mining activity trapped in the permafrost appear to enter the coastal environments as ground ice melts. Consequently, PAHs are currently emerging as the most significant contributors to potential risks in the Svalbard ecosystems.
引用
收藏
页数:10
相关论文
共 50 条
  • [41] Dry deposition of particulate polychlorinated biphenyls and polycyclic aromatic hydrocarbons to Lake Michigan
    Franz, TP
    Eisenreich, SJ
    Holsen, TM
    ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1998, 32 (23) : 3681 - 3688
  • [42] Accumulation of polychlorinated biphenyls and polycyclic aromatic hydrocarbons in the snowpack of Minnesota and Lake Superior
    Franz, TP
    Eisenreich, SJ
    JOURNAL OF GREAT LAKES RESEARCH, 2000, 26 (02) : 220 - 234
  • [43] Nanotechnology to remove polychlorinated biphenyls and polycyclic aromatic hydrocarbons from water: a review
    Borji, Hadil
    Ayoub, George M.
    Al-Hindi, Mahmoud
    Malaeb, Lilian
    Hamdan, Hamdan Z.
    ENVIRONMENTAL CHEMISTRY LETTERS, 2020, 18 (03) : 729 - 746
  • [44] Polycyclic aromatic hydrocarbons and polychlorinated biphenyls in urban soils from Kathmandu, Nepal
    Aichner, B.
    Glaser, B.
    Zech, W.
    ORGANIC GEOCHEMISTRY, 2007, 38 (04) : 700 - 715
  • [45] Distributions and potential sources of traditional and emerging polycyclic aromatic hydrocarbons in sediments from the lower reach of the Yangtze River, China
    Hong, Seongjin
    Kim, Youngnam
    Lee, Yeonjung
    Yoon, Seo Joon
    Lee, Changkeun
    Liu, Peng
    Kwon, Bong-Oh
    Hu, Wenyou
    Khim, Jong Seong
    SCIENCE OF THE TOTAL ENVIRONMENT, 2022, 815
  • [47] One century record of contamination by polycyclic aromatic hydrocarbons and polychlorinated biphenyls in core sediments from the southern Yellow Sea
    Zhang Peng
    Song Jinming
    Fang Jie
    Liu Zhigang
    Li Xuegang
    Yuan Huamao
    JOURNAL OF ENVIRONMENTAL SCIENCES, 2009, 21 (08) : 1080 - 1088
  • [48] One century record of contamination by polycyclic aromatic hydrocarbons and polychlorinated biphenyls in core sediments from the southern Yellow Sea
    ZHANG Peng SONG Jinming FANG Jie LIU Zhigang LI Xuegang YUAN Huamao Key Laboratory Marine Ecology and Environmental Sciences Institute of Oceanology Chinese Academy of Sciences Qingdao China The Graduate University of Chinese Academy of Sciences Beijing China Zhejiang Zhoushan Marine Ecological Environmental Monitoring Station Zhoushan China
    Journal of Environmental Sciences, 2009, 21 (08) : 1080 - 1088
  • [49] Effects of dose and particle size on activated carbon treatment to sequester polychlorinated biphenyls and polycyclic aromatic hydrocarbons in marine sediments
    Zimmerman, JR
    Werner, D
    Ghosh, U
    Millward, RN
    Bridges, TS
    Luthy, RG
    ENVIRONMENTAL TOXICOLOGY AND CHEMISTRY, 2005, 24 (07) : 1594 - 1601
  • [50] Presence, Sources and Transport of Polycyclic Aromatic Hydrocarbons in the Arctic Ocean
    Zhang, Lihong
    Ma, Yuxin
    Vojta, Simon
    Morales-McDevitt, Maya
    Hoppmann, Mario
    Soltwedel, Thomas
    Kirk, Jane
    De Silva, Amila
    Muir, Derek
    Lohmann, Rainer
    GEOPHYSICAL RESEARCH LETTERS, 2023, 50 (01)