A minireview on selected applications of in situ infrared spectroscopy in studying CO2 electrochemical reduction reaction

被引：14
|
作者：
Xu, Hongming [1 ,2 ]
Fan, Zhanxi [2 ]
Zhu, Shangqian [3 ]
Shao, Minhua [1 ,4 ]
机构：
[1] Hong Kong Univ Sci & Technol, Dept Chem & Biol Engn, Clear Water Bay, Hong Kong, Peoples R China
[2] City Univ Hong Kong, Dept Chem, Kowloon, Tat Chee Ave, Hong Kong, Peoples R China
[3] Southeast Univ, Sch Chem & Chem Engn, Nanjing 211189, Jiangsu, Peoples R China
[4] Hong Kong Univ Sci & Technol, Energy Inst, Kowloon, Clear Water Bay, Hong Kong, Peoples R China
来源：
CURRENT OPINION IN ELECTROCHEMISTRY | 2023年 / 41卷
关键词：
Electrochemical spectroscopy; Reaction mechanisms; Cation effects; Electrochemical interfaces; Carbon dioxide reduction; INTERNAL-REFLECTION; INTERMEDIATE; INTERFACE; CATIONS;
D O I：
10.1016/j.coelec.2023.101363
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
In situ infrared spectroscopy is a powerful tool to obtain molecular-level information of local environments and reaction mechanisms in solid-liquid electrochemical interfaces. The information gained by this technique can facilitate the rational design of more efficient electrocatalysts and electrochemical systems. In this minireview, two selected applications of in situ infrared spectroscopy in studying CO2 reduction reaction are presented, including the elucidations of the role of cations and the catalyst structure/composition-performance relationship. Some opinions on the future development of this technique are also provided.
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页数：8
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