Antiferromagnetic metal phase in an electron-doped rare-earth nickelate

被引:16
|
作者
Song, Qi [1 ]
Doyle, Spencer [1 ]
Pan, Grace A. [1 ]
El Baggari, Ismail [2 ]
Segedin, Dan Ferenc [1 ]
Carrizales, Denisse Cordova [1 ]
Nordlander, Johanna [1 ]
Tzschaschel, Christian [3 ]
Ehrets, James R. [1 ]
Hasan, Zubia [1 ]
El-Sherif, Hesham [2 ]
Krishna, Jyoti [4 ]
Hanson, Chase [4 ]
LaBollita, Harrison [4 ]
Bostwick, Aaron [5 ]
Jozwiak, Chris [5 ]
Rotenberg, Eli [5 ]
Xu, Su-Yang [3 ]
Lanzara, Alessandra [6 ,7 ]
N'Diaye, Alpha T. [5 ]
Heikes, Colin A. [8 ,9 ,10 ]
Liu, Yaohua [11 ,12 ]
Paik, Hanjong [13 ,14 ,15 ]
Brooks, Charles M. [1 ]
Pamuk, Betuel
Heron, John T. [16 ]
Shafer, Padraic [5 ]
Ratcliff, William D. [8 ]
Botana, Antia S. [4 ]
Moreschini, Luca [6 ,7 ,13 ]
Mundy, Julia A. [1 ]
机构
[1] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA
[2] Harvard Univ, Rowland Inst Harvard, Cambridge, MA USA
[3] Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA USA
[4] Arizona State Univ, Dept Phys, Tempe, AZ USA
[5] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA USA
[6] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
[7] Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA
[8] NIST, NIST Ctr Neutron Res, Gaithersburg, MD USA
[9] NIST, Joint Quantum Inst, Gaithersburg, MD USA
[10] Univ Maryland, Dept Mat Sci & Engn, Gaithersburg, MD USA
[11] Oak Ridge Natl Lab, Neutron Scattering Div, Oak Ridge, TN USA
[12] Oak Ridge Natl Lab, Target Stn 2, Oak Ridge, TN USA
[13] Cornell Univ, Platform Accelerated Realizat Anal & Discovery Int, Ithaca, NY 14850 USA
[14] Univ Oklahoma, Sch Elect & Comp Engn, Norman, OK USA
[15] Univ Oklahoma, Ctr Quantum Res & Technol CQRT, Norman, OK USA
[16] Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI USA
基金
美国国家科学基金会; 瑞士国家科学基金会;
关键词
INSULATOR-TRANSITION; RNIO3; R; HOLE;
D O I
10.1038/s41567-022-01907-2
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Long viewed as passive elements, antiferromagnetic materials have emerged as promising candidates for spintronic devices due to their insensitivity to external fields and potential for high-speed switching. Recent work exploiting spin and orbital effects has identified ways to electrically control and probe the spins in metallic antiferromagnets, especially in non-collinear or non-centrosymmetric spin structures. The rare-earth nickelate NdNiO3 is known to be a non-collinear antiferromagnet in which the onset of antiferromagnetic ordering is concomitant with a transition to an insulating state. Here we find that for low electron doping, the magnetic order on the nickel site is preserved, whereas electronically, a new metallic phase is induced. We show that this metallic phase has a Fermi surface that is mostly gapped by an electronic reconstruction driven by bond disproportionation. Furthermore, we demonstrate the ability to write to and read from the spin structure via a large zero-field planar Hall effect. Our results expand the already rich phase diagram of rare-earth nickelates and may enable spintronics applications in this family of correlated oxides. Films of the correlated oxide NdNiO3 form a metallic antiferromagnetic phase that can be identified using electrical currents, raising the prospect of applications in spintronics.
引用
收藏
页码:522 / +
页数:10
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