Long-term planetary boundary layer features and associated PM2.5 pollution anomalies in Beijing during the past 40 years

被引:6
|
作者
Yan, Yan [1 ]
Cai, Xuhui [1 ]
Huang, Qianqian [2 ]
Qi, Peng [3 ]
Song, Yu [1 ]
Zhang, Hongsheng [4 ]
Zeng, Limin [1 ]
机构
[1] Peking Univ, Coll Environm Sci & Engn, State Key Joint Lab Environm Simulat & Pollut Cont, Beijing 100871, Peoples R China
[2] China Meteorol Adm, Inst Urban Meteorol, Beijing 100089, Peoples R China
[3] China Meteorol Adm, Weather Modificat Ctr & Cloud Precipitat Phys, Weather Modificat Key Lab, Beijing 100081, Peoples R China
[4] Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Beijing 100871, Peoples R China
基金
中国国家自然科学基金;
关键词
PARTICULATE MATTER; AIR-QUALITY; SEVERE HAZE; METEOROLOGICAL CONDITIONS; AEROSOL POLLUTION; SYNOPTIC PATTERNS; PERSISTENT HAZE; EASTERN CHINA; WIND SHEAR; IMPACT;
D O I
10.1007/s00704-023-04356-w
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Primary work on the planetary boundary layer (PBL) climatic features and associated air pollution in Beijing was carried out based on a 40-year dataset. The main results are identified as follows. The annual mean PBL height was 906 m (1455 m in daytime and 357 m in nighttime). Within the PBL, the average potential temperature, specific humidity, and wind speed were 287.3 K, 5.1 g kg(-1), and 6.5 m s(-1). Significant seasonal variations were observed in the PBL variables, leading to distinct pollutant diffusion conditions. The PM2.5 concentrations varied seasonally, with a high value in winter (97 mu g m(-3)) and a low value in summer (74 mu g m(-3)). The summertime PM2.5 was closely related to the local emission intensity (R = 0.79) and declined with a reduction in the emission intensity, while the winter PM2.5 showed large interannual variabilities and trends, relying more on the PBL conditions. A comparison of polluted and clean winters was performed, revealing that polluted winters were associated with a warmer layer above the PBL that inhibited the development of the PBL (933 m vs. 1283 m, daily maximum height for polluted vs. clean winters) and led to a humid (1.4 g kg(-1) vs. 0.8 g kg(-1)) and weak wind (5.8 m s(-1) vs. 8.2 m s(-1)) layer within the PBL. In terms of synoptic impacts, the warm advection above the PBL (0.07 K h(-1)) and subsidence heating (0.21 K h(-1)) near the top of the PBL contributed to the occurrence of a stable and polluted PBL.
引用
收藏
页码:1787 / 1804
页数:18
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