Disordering two-dimensional magnet-particle configurations using bidispersity

被引:0
|
作者
Tsuchikusa, K. [1 ]
Yamamoto, K. [1 ,2 ]
Katsura, M. [1 ]
de Paula, C. T. [3 ]
Modesto, J. A. C. [3 ]
Dorbolo, S. [4 ]
Pacheco-Vazquez, F. [5 ]
Sobral, Y. D. [3 ]
Katsuragi, H. [1 ]
机构
[1] Osaka Univ, Dept Earth & Space Sci, 1 1 Machikaneyama, Toyonaka 5600043, Japan
[2] Tokyo Univ Sci, Water Frontier Res Ctr WaTUS, 6 3 1 Niijuku,Katsushika ku, Tokyo 1258585, Japan
[3] Univ Brasilia, Dept Matemat, Campus Univ Darcy Ribeiro, BR-70910900 Brasilia, DF, Brazil
[4] Univ Liege, Inst Phys Bldg B5a, GRASP, B-4000 Liege, Belgium
[5] Benemerita Univ Autonoma Puebla, Inst Fis, Apartado Postal J 48, Puebla 72570, Mexico
来源
JOURNAL OF CHEMICAL PHYSICS | 2023年 / 158卷 / 21期
关键词
CRYSTALS;
D O I
10.1063/5.0149803
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In various types of many-particle systems, bidispersity is frequently used to avoid spontaneous ordering in particle configuration. In this study, the relation between bidispersity and disorder degree of particle configuration is investigated. By using magnetic dipole-dipole interaction, magnet particles are dispersed in a two-dimensional cell without physical contact between them. In this magnetic system, bidispersity is introduced by mixing large and small magnets. Then, the particle system is compressed to produce a uniform particle configuration. The compressed particle configuration is analyzed by using Voronoi tessellation for evaluating the disorder degree which strongly depends on bidispersity. Specifically, standard deviation and skewness of the Voronoi cell area distribution are measured. As a result, we find that the peak of standard deviation is observed when the numbers of large and small particles are almost identical. Although the skewness shows non-monotonic behavior, zero skewness state (symmetric distribution) can be achieved when the numbers of large and small particles are identical. In this ideally random (disordered) state, the ratio between pentagonal, hexagonal, and heptagonal Voronoi cells become roughly identical, while hexagons are dominant in monodisperse (ordered) condition. The relation between Voronoi cell analysis and the global bond orientational order parameter is also discussed.
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页数:9
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