In-Situ Hydrothermal Synthesis of Ag3PO4/g-C3N4 Nanocomposites and Their Photocatalytic Decomposition of Sulfapyridine under Visible Light

被引:3
|
作者
Li, Ke [1 ,2 ,3 ]
Chen, Miaomiao [1 ]
Chen, Lei [1 ]
Zhao, Songying [1 ]
Xue, Wencong [1 ]
Han, Zixuan [1 ]
Han, Yanchao [2 ]
Zhang, Fuguo [3 ]
Yan, Yu [3 ]
Dong, Yanhong [3 ]
机构
[1] Jilin Jianzhu Univ, Key Lab Song Liao Aquat Environm, Minist Educ, Changchun 130118, Peoples R China
[2] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Peoples R China
[3] China Northeast Municipal Engn Design & Res Inst C, Changchun 130021, Peoples R China
基金
中国国家自然科学基金;
关键词
visible light; photocatalysis; Ag3PO4; g-C3N4; sulfapyridine; GRAPHITIC CARBON NITRIDE; FE-DOPED G-C3N4; HYBRID PHOTOCATALYSTS; ANTIBIOTIC POLLUTION; WATER OXIDATION; TREATMENT-PLANT; EFFICIENT; DEGRADATION; HETEROJUNCTION; FABRICATION;
D O I
10.3390/pr11020375
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Highly efficient visible-light-driven heterogeneous photocatalyst Ag3PO4/g-C3N4 with different weight ratios from Ag3PO4 to g-C3N4 were synthesized by a facile in situ hydrothermal method and characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), Fourier transform infrared spectrometry (FTIR), photoluminescence spectra (PL), UV-vis diffuse reflectance spectra (UV-Vis), and electrochemical impedance spectra (EIS). Under visible light irradiation, Ag3PO4/g-C3N4 showed very excellent photocatalytic activity for sulfapyridine (SP) which is one of the widely used sulfonamide antibiotics. When the ratio from Ag3PO4 to g-C3N4 was 1:2, the degradation rate of SP at 120 min was found to be 94.1%, which was superior to that of pure Ag3PO4 and pure g-C3N4. Based on the experimental results, the possible enhanced photocatalytic mechanism of Ag3PO4/g-C3N4 was proposed.
引用
收藏
页数:12
相关论文
共 50 条
  • [21] Synthesis of Ag3PO4/Ag/g-C3N4 Composite for Enhanced Photocatalytic Degradation of Methyl Orange
    Liu, Qingwang
    Meng, Ying
    Liu, Qiman
    Xu, Mai
    Hu, Yunhu
    Chen, Shikun
    MOLECULES, 2023, 28 (16):
  • [22] Synthesis and photocatalytic application of trinary structural g-C3N4/Ag/Ag3PO4 composite nanomaterials
    Liu, Jun
    Tian, Qingyong
    Wu, Zhaohui
    Yao, Weijing
    Xiao, Xiangheng
    Wu, Wei
    JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2017, 5 (06): : 5777 - 5785
  • [23] In-situ synthesis of CdS/g-C3N4 hybrid nanocomposites with enhanced visible photocatalytic activity
    Zhang L. Fang
    Huang F. Rong
    Zhou L. Ya
    Pang Qi
    Journal of Materials Science, 2015, 50 : 3057 - 3064
  • [24] In-situ synthesis of CdS/g-C3N4 hybrid nanocomposites with enhanced visible photocatalytic activity
    Fang, Zhang L.
    Rong, Huang F.
    Ya, Zhou L.
    Qi, Pang
    JOURNAL OF MATERIALS SCIENCE, 2015, 50 (08) : 3057 - 3064
  • [25] Photocatalytic degradation mechanism of phenanthrene over visible light driven plasmonic Ag/Ag3PO4/g-C3N4 heterojunction nanocomposite
    Dai, Yuxuan
    Wang, Yuting
    Zuo, Gancheng
    Kong, Jijie
    Guo, Yang
    Sun, Cheng
    Xian, Qiming
    CHEMOSPHERE, 2022, 293
  • [26] In situ synthesis of Ag3PO4/cellulose nanocomposites with photocatalytic activities under sunlight
    Wang, Qiyang
    Cai, Jie
    Zhang, Lina
    CELLULOSE, 2014, 21 (05) : 3371 - 3382
  • [27] In situ synthesis of Ag3PO4/cellulose nanocomposites with photocatalytic activities under sunlight
    Qiyang Wang
    Jie Cai
    Lina Zhang
    Cellulose, 2014, 21 : 3371 - 3382
  • [28] Photocatalytic Inactivation of Bacteriophage f2 with Ag3PO4/g-C3N4 Composite under Visible Light Irradiation: Performance and Mechanism
    Cheng, Rong
    Shen, Liang-jie
    Yu, Jin-hui
    Xiang, Shao-yu
    Zheng, Xiang
    CATALYSTS, 2018, 8 (10):
  • [29] Enhanced photocatalytic activity of ternary Ag3PO4/GO/g-C3N4 photocatalysts for Rhodamine B degradation under visible light radiation
    Yan, Jia
    Song, Zhilong
    Wang, Xin
    Xu, Yuanguo
    Pu, Wenjie
    Xu, Hui
    Yuan, Shouqi
    Li, Huaming
    APPLIED SURFACE SCIENCE, 2019, 466 : 70 - 77
  • [30] Photocatalytic degradation of bisphenol A by Ag3PO4 under visible light
    Katsumata, Hideyuki
    Taniguchi, Masanao
    Kaneco, Satoshi
    Suzuki, Tohru
    CATALYSIS COMMUNICATIONS, 2013, 34 : 30 - 34