In-Situ Hydrothermal Synthesis of Ag3PO4/g-C3N4 Nanocomposites and Their Photocatalytic Decomposition of Sulfapyridine under Visible Light

被引:3
|
作者
Li, Ke [1 ,2 ,3 ]
Chen, Miaomiao [1 ]
Chen, Lei [1 ]
Zhao, Songying [1 ]
Xue, Wencong [1 ]
Han, Zixuan [1 ]
Han, Yanchao [2 ]
Zhang, Fuguo [3 ]
Yan, Yu [3 ]
Dong, Yanhong [3 ]
机构
[1] Jilin Jianzhu Univ, Key Lab Song Liao Aquat Environm, Minist Educ, Changchun 130118, Peoples R China
[2] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Peoples R China
[3] China Northeast Municipal Engn Design & Res Inst C, Changchun 130021, Peoples R China
基金
中国国家自然科学基金;
关键词
visible light; photocatalysis; Ag3PO4; g-C3N4; sulfapyridine; GRAPHITIC CARBON NITRIDE; FE-DOPED G-C3N4; HYBRID PHOTOCATALYSTS; ANTIBIOTIC POLLUTION; WATER OXIDATION; TREATMENT-PLANT; EFFICIENT; DEGRADATION; HETEROJUNCTION; FABRICATION;
D O I
10.3390/pr11020375
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Highly efficient visible-light-driven heterogeneous photocatalyst Ag3PO4/g-C3N4 with different weight ratios from Ag3PO4 to g-C3N4 were synthesized by a facile in situ hydrothermal method and characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), Fourier transform infrared spectrometry (FTIR), photoluminescence spectra (PL), UV-vis diffuse reflectance spectra (UV-Vis), and electrochemical impedance spectra (EIS). Under visible light irradiation, Ag3PO4/g-C3N4 showed very excellent photocatalytic activity for sulfapyridine (SP) which is one of the widely used sulfonamide antibiotics. When the ratio from Ag3PO4 to g-C3N4 was 1:2, the degradation rate of SP at 120 min was found to be 94.1%, which was superior to that of pure Ag3PO4 and pure g-C3N4. Based on the experimental results, the possible enhanced photocatalytic mechanism of Ag3PO4/g-C3N4 was proposed.
引用
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页数:12
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