TiO2/Activated Carbon/2D Selenides Composite Photocatalysts for Industrial Wastewater Treatment

被引:5
|
作者
Ahmad, Shehzad [1 ]
Tahir, Muhammad Suleman [2 ,3 ]
Kamal, Ghulam Mustafa [1 ,4 ]
Zhang, Xu [5 ,6 ,7 ]
Nazir, Saima [4 ,8 ]
Tahir, Muhammad Bilal [9 ]
Jiang, Bin [5 ,6 ,7 ]
Safdar, Muhammad [1 ]
机构
[1] Khwaja Fareed Univ Engn & Informat Technol, Inst Chem, Rahim Yar Khan 64200, Pakistan
[2] Khwaja Fareed Univ Engn & Informat Technol, Inst Chem & Environm Engn, Rahim Yar Khan 64200, Pakistan
[3] Univ Gujrat, Dept Chem Engn, Gujrat 50700, Pakistan
[4] Khwaja Fareed Univ Engn & Informat Technol, Inst Hlth Sci, Rahim Yar Khan 64200, Pakistan
[5] Opt Valley Lab, Wuhan 430074, Peoples R China
[6] Chinese Acad Sci, Wuhan Inst Phys & Math, Innovat Acad Precis Measurement Sci & Technol, Natl Ctr Magnet Resonance Wuhan,Key Lab Magnet Res, Wuhan 430074, Peoples R China
[7] Huazhong Univ Sci & Technol, Wuhan Natl Lab Optoelect, Wuhan 430071, Peoples R China
[8] Univ Gujrat, Nawaz Sharif Med Coll, Gujrat 50700, Pakistan
[9] Khwaja Fareed Univ Engn & Informat Technol, Inst Phys, Rahim Yar Khan 64200, Pakistan
基金
中国国家自然科学基金;
关键词
TiO(2)activated carbon; 2D selenides; photocatalyst; wastewater treatment; GRAPHENE SAND COMPOSITE; TIO2; NANOPARTICLES; OPTICAL-PROPERTIES; DOPED TIO2; DEGRADATION; NANOTECHNOLOGY; MOS2; DYE; OXYTETRACYCLINE; MINERALIZATION;
D O I
10.3390/w15091788
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Even in the 21st century, water contamination has been a big problem and industrial processes are to be blamed for polluted water supplies. The use of sunlight in the process of photocatalysis is an efficientway to purifywastewater. Composites of TiO2/activated carbon/two-dimensional selenides performed better than either of the individual material or binary composites for this application. A straightforward hydrothermal technique was employed in the synthesis of photocatalysts. The synthesized photocatalytic composites were verified with the help of UV-Visible spectroscopy, FTIR, XRD, and SEM. The heterostructures absorbed nearly all of the sun's UV and visible light. These photons are then converted into usable reducing electrons and oxidizing species such as O-center dot(2) and OH center dot to decompose organic pollutants from industrial wastewater. Since there were additional pathways available for charge transfer along with several active edge sites, the composite photocatalysts are proven more active than individual TiO2 and 2D MoSe2 components. With the help of a cascadedriven mechanism of electrons, these channels can transmit more charges than single-component heterojunctions. The results provided a realistic method for developing photocatalyst composites powered by solar light for use in industrial wastewater treatment. Results of degradation of methylene blue suggest that the synthesized composites possess better photocatalytic activity. This enhanced photocatalytic activity is not limited to organic dyes. Other hazardous organic pollutants present in industrial wastewater can be decomposed by using this approach.
引用
收藏
页数:22
相关论文
共 50 条
  • [21] Preparation of magnesium aminoclay-carbon dots/TiO2 as photocatalysts for wastewater management
    Bui, Vu Khac Hoang
    Koh, Jin-Soo
    Lee, Hyun Uk
    Park, Duckshin
    Lee, Young-Chul
    MATERIALS CHEMISTRY AND PHYSICS, 2022, 290
  • [22] Preparation of TiO2 Composite Photocatalysts and their Photocatalytic Performance
    Zhao, Xiaoyu
    Wei, Ju
    Ge, Jiali
    Chang, Shuaicai
    Lin, Sucun
    Li, Hongyu
    JOURNAL OF MACROMOLECULAR SCIENCE PART B-PHYSICS, 2023, 62 (06): : 280 - 296
  • [23] Efficient photocatalysts by hydrothermal treatment of TiO2
    Kontos, AI
    Arabatzis, IM
    Tsoukleris, DS
    Kontos, AG
    Bernard, MC
    Petrakis, DE
    Falaras, P
    CATALYSIS TODAY, 2005, 101 (3-4) : 275 - 281
  • [24] 2D advanced materials and technologies for industrial wastewater treatment
    Choi, Myong Yong
    Theerthagiri, Jayaraman
    Maia, Gilberto
    CHEMOSPHERE, 2021, 284
  • [25] Wastewater treatment with the advent of TiO2 endowed photocatalysts and their reaction kinetics with scavenger effect
    Das, Ajit
    Adak, Mrinal K.
    Mahata, Nagendranath
    Biswas, Bhaskar
    JOURNAL OF MOLECULAR LIQUIDS, 2021, 338 (338)
  • [26] The role of carbon in the photocatalytic reaction of carbon/TiO2 photocatalysts
    Teng, Feng
    Zhang, Guozhi
    Wang, Youqing
    Gao, Caitian
    Chen, Lulu
    Zhang, Peng
    Zhang, Zhenxing
    Xie, Erqing
    APPLIED SURFACE SCIENCE, 2014, 320 : 703 - 709
  • [27] Synergistic adsorption and photocatalysis study of TiO2 and activated carbon composite
    Yue, Yihang
    Yue, Xiaoju
    Tang, Xiaofeng
    Han, Lin
    Wang, Jinnong
    Wang, Shifeng
    Du, Chun
    HELIYON, 2024, 10 (10)
  • [28] Photodegradation of Toluene by Composite Photocatalysts of Organobentonites and TiO2: Influences of Carbon Chain Length
    Chen, Xiasheng
    Chen, Kunyang
    Bai, Ge
    Liu, Jianlei
    Lin, Meijiao
    Shen, Xueyou
    FUNDAMENTAL OF CHEMICAL ENGINEERING, PTS 1-3, 2011, 233-235 : 1958 - +
  • [29] Composite photocatalysts based on TiO2 - carbon for air pollutant removal: Aspects of adsorption
    Krysa, J.
    Baudys, M.
    Vislocka, X.
    Neumann-Spallart, M.
    CATALYSIS TODAY, 2020, 340 (340) : 34 - 39
  • [30] Carbon modified TiO2 photocatalysts for water purification
    Morawski, Antoni W.
    Janus, Magdalena
    Tryba, Beata
    Toyoda, Masahiro
    Tsumura, Tomoki
    Inagaki, Michio
    POLISH JOURNAL OF CHEMICAL TECHNOLOGY, 2009, 11 (02) : 46 - 50