TiO2 sensitized by red-, green-, blue-emissive carbon dots for enhanced H2 production

被引:9
|
作者
Dong-Xue Yang [1 ]
Dan Qu [1 ]
Xiang Miao [1 ]
Wen-Shuai Jiang [1 ]
Li An [1 ]
Yuan-Jing Wen [1 ]
Dan-Dan Wu [1 ]
Zai-Cheng Sun [1 ]
机构
[1] Beijing Key Laboratory for Green Catalysis and Separation,Department of Chemistry and Chemical Engineering, School of Environmental and Energy, Beijing University of Technology
基金
中国国家自然科学基金; 北京市自然科学基金; 中国博士后科学基金;
关键词
TiO2; Carbon dots; Visible light absorption; Sensitizer; H2production;
D O I
暂无
中图分类号
O643.36 [催化剂]; TQ116.2 [氢气];
学科分类号
0817 ; 081705 ;
摘要
Carbon dots(Cdots) with a broad light absorption range could be a potential stable sensitizer for TiO,which is an excellent ultraviolet(UV) response photocatalyst. Herein, we systematically investigated the different color emissive Cdots-sensitized TiOfor Hproduction.Firstly, all kinds of Cdots enhanced the photocatalytic properties of TiO. All the Cdots-sensitized TiOexhibits visible light Hproduction due to their absorption in the visible light region. The photocurrent and Hproduction amount display strong dependence on the light absorption range of Cdots. The blue-emissive Cdots endow the weak Hproduction rate due to its weak absorption in the visible light. The enhanced photocatalytic activities are mainly contributed to the strong light absorbance and high-efficient charge separation. The light absorption of green-and red-emissive Cdots is another main factor for the high catalytic activities besides charge separation.
引用
收藏
页码:404 / 412
页数:9
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