Efficient Removal of Uranium (VI) by One-Step Synthetic Environmentally Friendly Hydroxyapatite Modified Attapulgite Composite Material: Adsorption Properties and Mechanism Studies

被引:3
|
作者
Li, Longxiang [1 ,2 ]
Zhou, Zhongkui [1 ,2 ]
Wang, Guanghui [1 ,2 ]
Guo, Yadan [1 ,2 ]
Zhang, Yishuo [1 ,2 ]
Xin, Yan [1 ,2 ]
Wei, Zhenzhen [1 ,2 ]
机构
[1] East China Univ Technol, State Key Lab Nucl Resources & Environm, Nanchang 330013, Jiangxi, Peoples R China
[2] East China Univ Technol, Jiangxi Prov Key Lab Genesis & Remediat Groundwate, Nanchang 330013, Jiangxi, Peoples R China
来源
WATER AIR AND SOIL POLLUTION | 2025年 / 236卷 / 01期
基金
中国国家自然科学基金;
关键词
Hydroxyapatite; Attapulgite; Environmentally friendly; Adsorption mechanism; Adsorption performance; Uranium; MIGRATION; KINETICS; U(VI);
D O I
10.1007/s11270-024-07651-y
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A one-step hydrothermal method was successfully employed to synthesize hydroxyapatite modified attapulgite composite material (HAP/ATP), which was characterized to determine physicochemical properties. Furthermore, the performance and mechanism of uranium removal by HAP/ATP were extensively investigated. Results indicated that HAP/ATP reached adsorption equilibrium for uranium at around 20 min with a maximum adsorption capacity of 387.27 mg<middle dot>g-1. Modern characterization techniques identified ion exchange, complexation, dissolution-precipitation, and electrostatic adsorption as the primary mechanisms for uranium removal by HAP/ATP. ATP, a type of clay mineral, possesses a large specific surface area and natural pores. When utilized as a carrier, ATP reduced agglomeration of load materials. HAP can introduce more adsorption functional groups for attapulgite, this is a synergy, exerting the complementarity of materials. HAP/ATP demonstrates promising potential as an environmentally friendly adsorbent material for the treatment of radioactive uranium-containing wastewater.
引用
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页数:16
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