FePt bimetallic nanoparticles: A highly efficient hydrogen evolution catalyst with tunable d-band center

被引:1
|
作者
Huang, Yue [1 ]
Chang, Shao-Zhong [1 ]
Zi, Tao-Qing [1 ]
Zhu, Lin [1 ]
Gao, Li [1 ,2 ]
Cao, Yan-Qiang [3 ]
Syed, Jawad Ali Shah [1 ]
Li, Wei-Min [1 ]
Wu, Di [1 ]
Li, Ai-Dong [1 ]
机构
[1] Nanjing Univ, Coll Engn & Appl Sci, Collaborat Innovat Ctr Adv Microstruct,Jiangsu Ke, Mat Sci & Engn Dept,Natl Lab Solid State Microstr, Nanjing 210093, Peoples R China
[2] Jiangsu Leadmicro Nanotechnol Co Ltd, Wuxi 214000, Peoples R China
[3] Nanjing Univ Sci & Technol, Sch Sci, Nanjing 210094, Peoples R China
关键词
Atoms - Bimetals - Iron alloys - Nanoparticles;
D O I
10.1063/5.0221952
中图分类号
O59 [应用物理学];
学科分类号
摘要
Atomic layer deposition-derived FePt alloy catalysts exhibit superb hydrogen evolution reaction (HER) activity under tuning of their composition, where the electronic structure is modulated by the ligand effect. We demonstrate that HER activity can be correlated with the calculated d-band center via a linear relationship.
引用
收藏
页数:6
相关论文
共 50 条
  • [31] Optimizing photocatalytic hydrogen evolution performance by rationally constructing S-scheme heterojunction to modulate the D-band center
    Jin, Zhiliang
    Yang, Cheng
    JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2025, 677 : 205 - 220
  • [32] Regulating the d-band center of Cu nanoparticles for efficient photo-driven catalytic CO2 reduction
    Wang, Libo
    Zhang, Shumin
    Zhang, Liuyang
    Yu, Jiaguo
    APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY, 2024, 355
  • [33] Tailoring the d-Band Centers Enables Co4N Nanosheets To Be Highly Active for Hydrogen Evolution Catalysis
    Chen, Zhiyan
    Song, Yao
    Cai, Jinyan
    Zheng, Xusheng
    Han, Dongdong
    Wu, Yishang
    Zang, Yipeng
    Niu, Shuwen
    Liu, Yun
    Zhu, Junfa
    Liu, Xiaojing
    Wang, Gongming
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2018, 57 (18) : 5076 - 5080
  • [34] Tuning the d-band center enables nickel-iron phosphide nanoprisms as efficient electrocatalyst towards oxygen evolution
    Zhang, Yi
    Xu, Jie
    Ding, Yigang
    Wang, Chundong
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2020, 45 (35) : 17388 - 17397
  • [35] Photocatalytic hydrogen evolution over nickel cobalt bimetallic phosphate anchored graphitic carbon nitrides by regulation of the d-band electronic structure
    Zhang, Yuanzheng
    Dai, Yunrong
    Yin, Lifeng
    Li, Huihui
    Chen, Xiang
    Chen, Bin
    CATALYSIS SCIENCE & TECHNOLOGY, 2020, 10 (11) : 3654 - 3663
  • [36] Ru nanoparticles supported on partially reduced TiO2 as highly efficient catalyst for hydrogen evolution
    Chen, Li-Na
    Wang, Su-Heng
    Zhang, Peng-Yang
    Chen, Zhi-Xin
    Lin, Xiao
    Yang, Hui-Juan
    Sheng, Tian
    Lin, Wen-Feng
    Tian, Na
    Sun, Shi-Gang
    Zhou, Zhi-You
    NANO ENERGY, 2021, 88
  • [37] Cu Nanoparticles Electrodeposited at Liquid-Liquid Interfaces: A Highly Efficient Catalyst for the Hydrogen Evolution Reaction
    Aslan, Emre
    Patir, Imren Hatay
    Ersoz, Mustafa
    CHEMISTRY-A EUROPEAN JOURNAL, 2015, 21 (12) : 4585 - 4589
  • [38] 3d-orbital overlap modulated d-band center of high-entropy oxyhydroxide for efficient oxygen evolution reaction
    Tang, Shaobing
    Shuang, Wei
    Wu, Yujun
    Jia, Zhichao
    Bai, Zhengyu
    Yang, Lin
    APPLIED SURFACE SCIENCE, 2025, 682
  • [39] The RuO2/NiRu heterogeneous interface optimizes the d-band center of the Ni-Ru catalyst for high-performance alkaline hydrogen evolution reaction
    Zhou, Yitian
    Liu, Yifan
    Tang, Hehua
    Lin, Bo-Lin
    JOURNAL OF MATERIALS CHEMISTRY A, 2023, 11 (20) : 10720 - 10726
  • [40] Bimetallic Ni-Pt nanoparticles immobilized on mesoporous N-doped carbon as a highly efficient catalyst for complete hydrogen evolution from hydrazine borane
    Wang, Wei
    Hong, Xiaoling
    Yao, Qilu
    Lu, Zhang-Hui
    JOURNAL OF MATERIALS CHEMISTRY A, 2020, 8 (27) : 13694 - 13701