Comprehensive analysis and risk assessment of fine road dust in Abbottabad city (Pakistan) with heavy traffic for potentially toxic elements

被引:2
|
作者
Jadoon, Waqar Azeem [1 ]
Khan, Yousaf Ali [2 ]
Varol, Memet [3 ]
Onjia, Antonije [4 ]
Mohany, Mohamed [5 ]
机构
[1] Hazara Univ Mansehra, Dept Earth & Environm Sci, Mansehra 21130, Pakistan
[2] Hazara Univ Mansehra, Dept Math & Stat, Mansehra 21130, Pakistan
[3] Malatya Turgut Ozal Univ, Agr Fac, Aquaculture Dept, Malatya, Turkiye
[4] Univ Belgrade, Fac Technol & Met, Karnegijeva 4, Belgrade 11120, Serbia
[5] King Saud Univ, Coll Pharm, Dept Pharmacol & Toxicol, POB 55760, Riyadh 11451, Saudi Arabia
关键词
Fine road dust; PTEs; Traffic pollution; APCS-MLR; Health risk assessment; Abbottabad; Pakistan; METAL CONTAMINATION; TRACE-ELEMENTS; HEALTH-HAZARDS; SOILS; APPORTIONMENT; SIALKOT;
D O I
10.1016/j.jhazmat.2024.136788
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Human activities have far-reaching impact on natural ecosystems, causing increasing disturbances and disruptions to the delicate balance of the environment. Poor land use planning, urbanization, infrastructure development, and unplanned tourism exacerbate contamination and degradation in tourist destinations, yet the pollution of potentially toxic elements (PTEs) in these environments remains inadequately explored. To address this issue, we investigated the concentrations of acid-digested PTEs in road dust in Abbottabad city (Pakistan) with heavy traffic. The current study also evaluated PTE associated pollution, ecological and health risks, and potential sources of these elements. The average concentrations (in mg kg-1) of PTEs in road dust were highest for Fe (15540), followed by Mn (304), Zn (139), Cu (50.0), Pb (21.5), Cr (13.0), Ni (10.3), Co (6.66), and Cd (0.236). The levels of Co, Cr, Mn, Ni, and Fe were below the upper continental crust (UCC) averages, while Cd, Cu, Pb, and Zn exceeded them. Spatially, Cd, Cu, Pb, and Zn were found at higher levels near traffic hotspots, bus stands and automobile workshops. Road dust in Abbottabad exhibited unpolluted to moderate pollution levels (geo accumulation index), with Cd, Cu, Zn, and Pb at 23 % of the sites. The enrichment factor results indicated a significant anthropogenic influence, with Cd being significantly enriched and Zn, Cu, and Pb moderately enriched. The contamination factor results revealed moderate contamination by (Cd: 2.62, Zn: 2.08, Cu: 1.79, Pb: 1.27). Single metal risk index showed that 61 % of the sites posed considerable to very high ecological risks due to Cd, which was highlighted as a significant concern. The absolute principal component scores-multiple linear regression model identified three factors contributing to PTE pollution: lithogenic (Co, Fe, Mn, Ni), traffic-related (Cd, Cu, Pb, Zn), and mixed sources (Cr), with contributions of 52.8 %, 35.8 %, and 11.4 %, respectively. The PTE hazard quotient and total hazard index values for children and adults were below the safe risk level of 1, indicating no non-carcinogenic health risks. The cumulative carcinogenic risk values to the residents were also within acceptable limits. However, children's susceptibility to non-carcinogenic risks is higher due to their behavior and lower body weight. This study highlights the accumulation of PTEs in Abbottabad's environment, which poses challenges to long-term sustainability, particularly amid unplanned tourism. Therefore, urgent measures are necessary to mitigate PTE pollution and preserve tourist spots and public health.
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页数:13
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