Characteristics of vertical Distribution and Environmental Factors of Antibiotics in Quaternary Sedimentary Column in Urban Areas

被引：0
|
作者：
Liu K. [1 ]
Tong L. [1 ,2 ,3 ]
Gan C. [1 ]
Wang Y.-W. [1 ]
Zhang J.-Y. [1 ]
He J. [4 ]
机构：
[1] School of Environmental Studies, China University of Geosciences, Wuhan
[2] State Environmental Protection Key Laboratory of Source Apportionment and Control of Aquatic Pollution, Ministry of Ecology and Environment, Wuhan
[3] Hubei Key Laboratory of Yangtze Catchment Environmental Aquatic Science, Wuhan
[4] Wuhan Geological Survey Center, China Geological Survey, Wuhan
来源：
Huanjing Kexue/Environmental Science | 2024年 / 45卷 / 01期
关键词：
antibiotics; borehole sediments; environmental factors; metals; vertical distribution;
D O I：
10.13227/j.hjkx.202212170
中图分类号：
学科分类号：
摘要：
Antibiotics easily remain in sediments after migrating from the surface to the subsurface due to water-rock interactions，posing a risk of secondary release to groundwater. To investigate the vertical distribution characteristics and environmental impact factors of antibiotics，five 30 m quaternary sediment columns were drilled and stratified near the hospital，and five major classes of antibiotics and sulfonamide metabolites were tested and analyzed. The results showed that：1 the antibiotic content in the sediments ranged from 3. 05 to 107. 03 μg·kg-1，and all of the target antibiotics were detected except lomefloxacin，of which ofloxacin and oxytetracycline were the most important antibiotics in the study area. 2 The antibiotics did not show a strict downward trend in the vertical direction but varied with the lithological stratification. 3 Antibiotics were primarily deposited in the clay layer and varied with the fluctuation of the groundwater level. 4 The results of redundancy analysis between antibiotics and environmental factors suggested that pH and TOC controlled the fate and transformation of antibiotics through influencing the adsorption of antibiotics by sediments. The risk of antibiotic contamination from hospital wastewater seepage into the subsurface environment should be taken seriously. © 2024 Science Press. All rights reserved.
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页码：584 / 593
页数：9
相关论文
共 45 条
  • [41] Zhao K，, Gao L，, Zhang Q R，, Et al., Accumulation of sulfamethazine and ciprofloxacin on grain surface decreases the transport of biochar colloids in saturated porous media［J］, Journal of Hazardous Materials, (2021)
  • [42] Hari A C，, Paruchuri R A，, Sabatini D A，, Et al., Effects of pH and cationic and nonionic surfactants on the adsorption of pharmaceuticals to a natural aquifer material［J］, Environmental Science & Technology, 39, 8, pp. 2592-2598, (2005)
  • [43] Wang C H，, Liang W，, Xue A F，, Et al., Advances on the performance of veterinary antibiotics in soil ［J］, Journal of Huazhong Agricultural University, 29, 2, pp. 245-250, (2010)
  • [44] Wang Y J, Jia D A，, Sun R J，, Et al., Adsorption and cosorption of tetracycline and copper（ II ） on montmorillonite as affected by solution pH［J］, Environmental Science & Technology, 42, 9, pp. 3254-3259, (2008)
  • [45] Figueroa R A, MacKay A A., Sorption of oxytetracycline to iron oxides and iron oxide-rich soils［J］, Environmental Science & Technology, 39, 17, pp. 6664-6671, (2005)
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