Long-Term Stability and Efficiency of VO2 Nanostructure-Based Thermochromic Smart Windows

被引:3
|
作者
Liang, Zihui [1 ]
Liao, Xiaohong [1 ]
Yu, Jing [4 ,5 ]
Zhou, Zezhu [2 ]
Wang, Hao [2 ]
Zhang, Teng [3 ]
Yi, Changhai [1 ]
Zhao, Li [2 ]
Chen, Fengxiang [1 ]
Wu, Congcong [2 ]
机构
[1] Wuhan Text Univ, Natl Local Joint Lab Adv Text Proc & Clean Prod, State Key Lab New Text Mat & Adv Proc Technol, Wuhan 430200, Peoples R China
[2] Hubei Univ, Key Lab Green Preparat & Applicat Funct Mat, Hubei Key Lab Polymer Mat, Minist Educ, Wuhan 430062, Peoples R China
[3] Hubei Minzu Univ, Coll Intelligent Syst Sci & Engn, Enshi 445000, Hubei, Peoples R China
[4] Huanjiang Lab, Zhuji 311800, Peoples R China
[5] Zhejiang Police Vocat Acad, Hangzhou 310018, Peoples R China
基金
中国国家自然科学基金;
关键词
Thermochromic; vanadium dioxide; phase transformation; smart windows; solar energy modulation; FILMS; PERFORMANCE; COATINGS;
D O I
10.1021/acsanm.4c03595
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Buildings, accounting for approximately 40% of global energy consumption, heavily rely on windows for maintaining indoor comfort. However, conventional windows are known for their inefficiency due to high optical transmittance and thermal conductivity. In recent decades, efforts have focused on enhancing sustainability through the development of low-emissivity coatings and smart windows. Despite advancements, the commercialization of a vanadium dioxide (VO2) nanostructure-based thermochromic film has been limited by stability issues. This study addresses the critical need for long-term stability and efficiency in VO2-based smart windows, showcasing a composite film that is highly resilient to heat, ultraviolet (UV) light, and humidity. The proposed films exhibit exceptional solar energy regulation capability (Delta T-sol = 20.11%) alongside a visible light transmittance of 54.94%. Moreover, they exhibit strong stability even under conditions of high relative humidity (90%) and temperature (60 degrees C), maintaining consistent phase-transition performance over 40 days & horbar;equivalent to approximately 1777 days of real-world exposure. Impressively, even without encapsulation, the composite film retains 96.4% of its initial Delta T-sol after continuous 60-day illumination. This research offers promising technical solutions for advancing the commercial viability of traditional VO2 smart windows, contributing significantly to global efforts toward carbon neutrality and sustainable development.
引用
收藏
页码:21683 / 21691
页数:9
相关论文
共 50 条
  • [31] Sn-W Co-doping Improves Thermochromic Performance of VO2 Films for Smart Windows
    Zhao, Zhengjing
    Liu, Yi
    Yu, Zhinong
    Ling, Chen
    Li, Jingbo
    Zhao, Yongjie
    Jin, Haibo
    ACS APPLIED ENERGY MATERIALS, 2020, 3 (10) : 9972 - 9979
  • [32] Microstructural Investigations of VO2 Thermochromic Thin Films Grown by Pulsed Laser Deposition for Smart Windows Applications
    Rai, Ayushi
    Iacob, Nicusor
    Leca, Aurel
    Locovei, Claudiu
    Kuncser, Victor
    Mihailescu, Cristian N.
    Delimitis, Andreas
    INORGANICS, 2022, 10 (12)
  • [33] VO2(M)@CeO2 core-shell nanospheres for thermochromic smart windows and photocatalytic applications
    Saini, Meenu
    Dehiya, Brijnandan S.
    Umar, Ahmad
    CERAMICS INTERNATIONAL, 2020, 46 (01) : 986 - 995
  • [34] Facile fabrication of VO2/SiO2 aerogel composite films with excellent thermochromic properties for smart windows
    Kang, Jiahong
    Liu, Jingxiao
    Shi, Fei
    Dong, Yutong
    Song, Xiaoying
    Wang, Zixuan
    Tian, Ziwei
    Xu, Jing
    Ma, Jing
    Zhao, Xinran
    APPLIED SURFACE SCIENCE, 2022, 573
  • [35] The improvement of bilayer VO2/TaOx thermochromic properties for smart window
    Dan-ke Chen
    Mao-ze Yu
    Chen-yang Hao
    Wei Mi
    Meng Wang
    Li-wei Zhou
    Jin-shi Zhao
    Journal of Materials Science: Materials in Electronics, 2022, 33 : 24734 - 24740
  • [36] The improvement of bilayer VO2/TaOx thermochromic properties for smart window
    Chen, Dan-ke
    Yu, Mao-ze
    Hao, Chen-yang
    Mi, Wei
    Wang, Meng
    Zhou, Li-wei
    Zhao, Jin-shi
    JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2022, 33 (32) : 24734 - 24740
  • [37] The potential cytotoxicity and mechanism of VO2 thin films for intelligent thermochromic windows
    Zhou, Huaijuan
    Li, Jinhua
    Bao, Shanhu
    Wang, Donghui
    Liu, Xuanyong
    Jin, Ping
    RSC ADVANCES, 2015, 5 (129) : 106315 - 106324
  • [38] Tungsten doped M-phase VO2 mesoporous nanocrystals with enhanced comprehensive thermochromic properties for smart windows
    Li, Bin
    Tian, Shouqin
    Tao, Haizheng
    Zhao, Xiujian
    CERAMICS INTERNATIONAL, 2019, 45 (04) : 4342 - 4350
  • [39] High-throughput roll-to-roll fabrication of flexible thermochromic coatings for smart windows with VO2 nanoparticles
    Kim, Youngkwang
    Yu, Sangbae
    Park, Jaeseoung
    Yoon, Daseob
    Dayaghi, Amir Masoud
    Kim, Kun Joong
    Ahn, Jin Soo
    Son, Junwoo
    JOURNAL OF MATERIALS CHEMISTRY C, 2018, 6 (13) : 3451 - 3458
  • [40] The synergistic effect of Ta-doping and antireflective TaOx layer on the thermochromic VO2 thin films for smart windows
    Sun, Hongli
    Chen, Danke
    Zhou, Liwei
    Mi, Wei
    Wang, Di
    He, Linan
    Zhao, Jinshi
    SOLAR ENERGY MATERIALS AND SOLAR CELLS, 2024, 275