Impacts of land cover changes on summer surface ozone in China during 2000-2019

被引:1
|
作者
Cao, Yang [1 ]
Yue, Xu [2 ]
Liao, Hong [2 ]
Wang, Xuemei [3 ]
Lei, Yadong [4 ,5 ]
Zhou, Hao [6 ]
机构
[1] Jiangsu Nanjing Environm Monitoring Ctr, Nanjing 210041, Peoples R China
[2] Nanjing Univ Informat Sci & Technol NUIST, Jiangsu Collaborat Innovat Ctr Atmospher Environm, Sch Environm Sci & Engn, Jiangsu Key Lab Atmospher Environm Monitoring & Po, Nanjing 210044, Peoples R China
[3] Jinan Univ, Inst Environm & Climate Res, Guangzhou 511443, Peoples R China
[4] Chinese Acad Meteorol Sci, State Key Lab Severe Weather, Beijing 100081, Peoples R China
[5] Chinese Acad Meteorol Sci, Key Lab Atmospher Chem CMA, Beijing 100081, Peoples R China
[6] Natl Univ Def Technol, Coll Meteorol & Oceanog, Changsha 410073, Peoples R China
关键词
Surface ozone; Land cover changes; Isoprene; Dry deposition; Forestation; ANTHROPOGENIC EMISSIONS; AIR-QUALITY; TROPOSPHERIC OZONE; ISOPRENE EMISSIONS; DRY DEPOSITION; GEOS-CHEM; VEGETATION; POLLUTION; CLIMATE; MODEL;
D O I
10.1016/j.scitotenv.2024.174821
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
China implemented continuous forestation and experienced significant greening tendency in the past several decades. While the ecological project brings benefits to regional carbon assimilation, it also affects surface ozone (O3) 3 ) pollution level through perturbations in biogenic emissions and dry deposition. Here, we use a coupled chemistry-vegetation model to assess the impacts of land use and land cover change (LULCC) on summertime surface O3 3 in China during 2000-2019. The LULCC is found to enhance O3 3 by 1-2 ppbv in already-polluted areas. In contrast, moderate reductions of-0.4 to-0.8 ppbv are predicted in southern China where the largest forest cover changes locate. Such inconsistency is attributed to the background chemical regimes with positive O3 3 changes over VOC-limited regions but negative changes in NOx-limited x-limited regions. The net contribution of LULCC to O3 3 budget in China is 24.17 Kg/s, in which the positive contribution by more isoprene emissions almost triples the negative effects by the increased dry deposition. Although the LULCC-induced O3 3 perturbation is much lower than the effects of anthropogenic emissions, forest expansion has exacerbated regional O3 3 pollution in North China Plain and is expected to further enhance surface O3 3 with continuous forestation in the future.
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页数:9
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