We numerically and analytically study ionization of H-2(+) with large internuclear distances R in strong elliptically polarized laser fields. Numerical simulations show that the offset angle in the photoelectron momentum distribution (PMD) is larger for cases of large R than for cases of H-2(+) with small R and model atoms with similar ionization potentials. In addition, the PMDs for cases of large R show clear interference patterns which disappear for cases of small R. By developing a strong-field model which includes the contributions of the first excited state and the Coulomb potential, we reproduce the phenomena for large R. Tunneling ionization of H-2(+) with large R involves a complex four-body interaction between the laser, the electron, and the two nuclei. Our model can approximate the four-body interaction as the three-body one and clearly identify the effects of charge resonance and different nuclei on tunneling ionization. Our work suggests a manner for probing complex interactions in strong-field ionization of stretched molecules with high time resolution.
机构:
Univ Szeged, Dept Theoret Phys, Tisza L Krt 84-86, H-6720 Szeged, HungaryUniv Szeged, Dept Theoret Phys, Tisza L Krt 84-86, H-6720 Szeged, Hungary
Majorosi, Szilard
Benedict, Mihaly G.
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Univ Szeged, Dept Theoret Phys, Tisza L Krt 84-86, H-6720 Szeged, HungaryUniv Szeged, Dept Theoret Phys, Tisza L Krt 84-86, H-6720 Szeged, Hungary
Benedict, Mihaly G.
Czirjak, Attila
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Univ Szeged, Dept Theoret Phys, Tisza L Krt 84-86, H-6720 Szeged, Hungary
ELI HU Nonprofit Ltd, ELI ALPS, Dugon Ter 13, H-6720 Szeged, HungaryUniv Szeged, Dept Theoret Phys, Tisza L Krt 84-86, H-6720 Szeged, Hungary
机构:
Kansas State Univ, Dept Phys, Manhattan, KS 66506 USA
Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USAKansas State Univ, Dept Phys, Manhattan, KS 66506 USA