Single-crystal neutron diffraction study on the Ho 13.6 Au 61.1 Al 25.3 quasicrystal approximant

被引:3
|
作者
Thilakan, Karthika K. [1 ]
Denoel, Fernand [2 ]
Huang, Yu-Chin [1 ]
Fabelo, Oscar [3 ]
Mathieu, Roland [2 ]
Gomez, Cesar Pay [1 ]
Sahlberg, Martin [1 ]
机构
[1] Uppsala Univ, Dept Chem, Angstrom Lab, S-75121 Uppsala, Sweden
[2] Uppsala Univ, Dept Mat Sci & Engn, Box 35, S-75103 Uppsala, Sweden
[3] Inst Laue Langevin, 71 Ave Martyrs,CS 20156, F-38042 Grenoble, France
关键词
Quasicrystal approximants; Magnetism; Neutron diffraction;
D O I
10.1016/j.jallcom.2024.175263
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A single-crystal neutron diffraction study was conducted on a Ho13.6Au61.1Al25.3 Tsai-type quasicrystal approximant synthesised by the self-flux method. The magnetisation measurements reveal a ferrimagnetic behaviour with a transition below 6 K. In agreement with the magnetometry data, a non-coplanar whirling spin order in the icosahedral clusters around the crystallographic [1 1 1] direction with a ferrimagnetic arrangement was observed from single-crystal neutron diffraction measurements below 5.5 K. The magnetic structure of Ho13.6Au61.1Al25.3 is compared to the previously published magnetic structures of related RE-Au-SM (RE = Tb and Ho; SM = Al, Si and Ga) systems.
引用
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页数:6
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