Optimization of nanoparticles transport model in porous media

被引:0
|
作者
Peng A. [1 ]
Zhan J. [1 ]
Wu M. [1 ]
机构
[1] School of Ocean Science and Technology, Dalian University of Technology, Panjin
来源
Huagong Xuebao/CIESC Journal | 2021年 / 72卷 / 10期
关键词
Model; Particle; Particle transport; Pore; Porous media;
D O I
10.11949/0438-1157.20210374
中图分类号
学科分类号
摘要
At present, the transport of nanoparticles in porous media such as soil is mostly described by a single-collector removal efficiency (η). However, this efficiency only considers the collecting effect of a single solid matrix, and does not consider the trapping effect of the pore space between the porous media such as T - E model. To address this issue, the water retention capacity (fr) was employed to reflect the number of small pores and the existing T-E model was modified. Research has shown that the transport of nanoparticles through columns with the same porosity (f) is not the same, but inversely proportional to the water retention capacity, which has been neglected in previous research. On this basis, the collector contact efficiency by the interception mechanism (ηI) is adjusted to be dependent on both porosity (f) and water retention capacity (fr); thus, the original model was optimized. Furthermore, breakthrough experiments on nanoscale silica particles (nSiO2) through the sand column and breakthrough experiments on nano titanium dioxide (nTiO2) through the sand column with different particle sizes proved that the optimized model is applicable to porous media with different particle sizes and is more accurate in predicting the transport of nanoparticles in porous media. © 2021, Editorial Board of CIESC Journal. All right reserved.
引用
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页码:5114 / 5122
页数:8
相关论文
共 30 条
  • [11] Swift D L, Friedlander S K., Coagulation of hydrosols by Brownian motion + laminar shear flow, Journal of Colloid Science, 19, 7, (1964)
  • [12] Logan B E, Jewett D G, Arnold R G, Et al., Clarification of clean-bed filtration models, Journal of Environmental Engineering, 121, 12, pp. 869-873, (1995)
  • [13] Yao K M, Habibian M T, O'Melia C R., Water and waste water filtration. Concepts and applications, Environmental Science & Technology, 5, 11, pp. 1105-1112, (1971)
  • [14] Ma H L, Hradisky M, Johnson W P., Extending applicability of correlation equations to predict colloidal retention in porous media at low fluid velocity, Environmental Science & Technology, 47, 5, pp. 2272-2278, (2013)
  • [15] Nelson K E, Ginn T R., New collector efficiency equation for colloid filtration in both natural and engineered flow conditions, Water Resources Research, 47, 5, (2011)
  • [16] Long W, Hilpert M., A correlation for the collector efficiency of Brownian particles in clean-bed filtration in sphere packings by a lattice-Boltzmann method, Environmental Science & Technology, 43, 12, pp. 4419-4424, (2009)
  • [17] Tufenkji N, Elimelech M., Breakdown of colloid filtration theory: role of the secondary energy minimum and surface charge heterogeneities, Langmuir, 21, 3, pp. 841-852, (2005)
  • [18] Rajagopalan R, Tien C., Trajectory analysis of deep-bed filtration with the sphere-in-cell porous media model, AIChE Journal, 22, 3, pp. 523-533, (1976)
  • [19] Tufenkji N, Elimelech M., Correlation equation for predicting single-collector efficiency in physicochemical filtration in saturated porous media, Environmental Science & Technology, 38, 2, pp. 529-536, (2004)
  • [20] Tufenkji N, Miller G F, Ryan J N, Et al., Transport of cryptosporidium oocysts in porous media: role of straining and physicochemical filtration, Environmental Science & Technology, 38, 22, pp. 5932-5938, (2004)