Electronic Spin Qubit Candidates Arrayed within Layered Two-Dimensional Polymers

被引：0

作者：

Oanta, Alexander K. ^{[1
]}

Collins, Kelsey A. ^{[1
]}

Evans, Austin M. ^{[1
]}

Pratik, Saied Md ^{[2
]}

Hall, Lyndon A. ^{[5
]}

Strauss, Michael J. ^{[1
]}

Marder, Seth R. ^{[3
,4
]}

D'Alessandro, Deanna M. ^{[5
]}

Rajh, Tijana ^{[6
,7
]}

Freedman, Danna E. ^{[1
,8
]}

Li, Hong ^{[2
]}

Brédas, Jean-Luc ^{[2
]}

Sun, Lei ^{[6
]}

Dichtel, William R. ^{[1
]}

机构：

[1] Department of Chemistry, Northwestern University, Evanston,IL,60208, United States

[2] Department of Chemistry and Biochemistry, The University of Arizona, Tucson,AZ,85721, United States

[3] School of Chemistry and Biochemistry, School of Materials Science and Engineering, Center for Organic Photonics and Electronics, Georgia Tech Polymer Network, Georgia Institute of Technology, Atlanta,GA,30332, United States

[4] Department of Chemistry, Renewable and Sustainable Energy Institute, University of Colorado Boulder, Boulder,CO,80303, United States

[5] School of Chemistry, The University of Sydney, Sydney,NSW,2006, Australia

[6] Center for Nanoscale Materials, Argonne National Laboratory, Lemont,IL,60439, United States

[7] The School of Molecular Sciences, Arizona State University, Tempe,AZ,85281, United States

[8] Department of Chemistry, Massachusetts Institute of Technology, Cambridge,MA,02139, United States

来源：

Journal of the American Chemical Society | 2023年 / 145卷 / 01期

关键词：

The Army Research Office is thanked for a Multidisciplinary University Research Initiative (MURI) award under grant W911NF-15-1-0447; which supported the preparation of electroactive 2DPs; characterization; and study using density functional theory. The Department of Energy grant DE-SC0019356 is thanked for supporting efforts at controlled molecular doping; including the investigation of charge transport; electronic structure; and paramagnetic behavior. A.M.E. (DGE-1324585); K.A.C; (DGE-1842165); and M.J.S. (DGE-11842165) were supported by the National Science Foundation Graduate Research Fellowship. A.M.E. is supported by the Schmidt Science Fellows; in partnership with the Rhodes Trust. L.S. was supported by the Laboratory Directed Research and Development (LDRD) funding from Argonne National Laboratory; provided by the Director; Office of Science; of the U.S. Department of Energy under Contract DE-AC02-06CH11357. D.M.D. (ARC FT170100283) gratefully acknowledges the Australian Research Council for funding. Dr. Nicholas Shepherd (University of Sydney) is kindly acknowledged for preliminary electrochemical and UV–vis–NIR spectroelectrochemical measurements. This study made use of IMSERC at Northwestern University; which has received support from the Soft and Hybrid Nanotechnology Experimental (SHyNE) Resource (NSF NNCI-1542205); the Materials Research Science and Engineering Center (National Science Foundation DMR-1720139); the State of Illinois; and the International Institute for Nanotechnology (IIN). Portions of this work were performed at the DuPont-Northwestern-Dow Collaborative Access Team (DND-CAT) located at Sector 5 and Sector 8 of the Advanced Photon Source (APS). DND-CAT was supported by Northwestern University; E.I. DuPont de Nemours & Co; and the Dow Chemical Company. This research used resources of the Advanced Photon Source and Center for Nanoscale Materials; both U.S. Department of Energy (DOE) Office of Science User Facilities operated for the DOE Office of Science by Argonne National Laboratory under contract DE-AC02-06CH11357; and the National Energy Research Scientific Computing Center; a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. Resources at the Advanced Photon Source were funded by National Science Foundation under award 0960140. The views expressed in the article do not necessarily represent the views of the DOE or the U.S. government. The U.S. government retains; and the publisher; by accepting the article for publication; acknowledges that the U.S. government retains a nonexclusive; paid-up; irrevocable; worldwide license to publish or reproduce the published form of this work; or allow others to do so; for U.S. government purposes;

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页码：689 / 696

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