SINGLE-ELECTRON TRANSFER IN ORGANIC-MOLECULES

被引：2

作者：

MALINSKY, J ^{[1
]}

MAGARSHAK, Y ^{[1
]}

SMOLYAR, A ^{[1
]}

LIPMAN, A ^{[1
]}

机构：

[1] CUNY MT SINAI SCH MED,DEPT PHYSIOL & BIOPHYS,NEW YORK,NY 10029

来源：

JOURNAL OF CHEMICAL PHYSICS | 1993年 / 98卷 / 05期

关键词：

D O I：

10.1063/1.464024

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The rate of electron transfer was studied in typical organic molecules. The approach is based on a Green's function technique which allows one to account for multiscattering electron tunneling. Quantum-chemical calculations are used to obtain the parameters of dynamical Dyson's equations for relevant double-time retarded Green's function. The parameters are used to estimate electron tunneling rate including neutral and mononegative ions of the alpha, omega-diphenylalkanes with different numbers of methyl groups. The role of bridge as the conductor of an extra electron is demonstrated from results of the calculations.

引用

页码：3968 / 3971

页数：4

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