Naturalism is a core component of S.T. Coleridge's romantic theology, where he expresses his understanding of the Universe, Nature and Life. His romantic philosophy explores God's influence in Heaven, on Earth, and on Man. From a tniquely romantic theological perspective, Coleridge expounds on Man's position in Nature, the human condition, and Man's relationship with God. The loss and recovery of the mysterious relationship between Man and Nature runs through all of his poetry and other writings. In his opinion, the mysterious relationship between Man and Nature could only be observed and expressed by imagination and symbolism, so he pours out his theological conceptions in a riotous profusion of poetic imagery. Hence, his work opens up a novel and interesting area of interdisciplinary research for the fields of theology and literature. This article tries to explore Coleridge's unique way of communicating theological concepts. He uses "moonlight" or " homeland in the moonlight" to portray notions of God's love, the home, or the hometown. He uses "eddy-rose" to symbolize the relationship between Man and God, Man and Nature, and Man's own destiny. He uses "intellectual breeze" to represent the absolute will of God, from which he analyzes the dilemma of man as he yearns for the unreachable home: under compulsion, Man in Nature, eddying in the breeze, longs for flight. Coleridge applauds Man's deep desire to become one with Nature even as the " intellectual breeze" blows. In showing how these imageries convey Coleridge's theological concepts, the paper traces the contours of naturalism in his romantic theological thought.