AN INTERPRETATION OF MOLECULAR FRAGMENTATION DYNAMICS IN TERMS OF THE RESONANCE-SPECTRUM

被引：7
|
作者：
JOLICARD, G [1 ]
ATABEK, O [1 ]
机构：
[1] UNIV PARIS 11,PHOTOPHYS MOLEC LAB,F-91405 ORSAY,FRANCE
来源：
JOURNAL OF CHEMICAL PHYSICS | 1990年 / 93卷 / 07期
关键词：
D O I：
10.1063/1.458665
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Quasidegenerate perturbation theory using a Bloch wave operator formalism is applied to the calculation of the rich resonance spectrum of a model polyatomic molecule undergoing photodissociation. The sharp structures (peaks and dips patterns) of the total dissociation rate as well as the partial probabilities to obtain the fragments at given internal states for various incident photon energies, are interpreted in terms of tunneling, shape or Feshbach resonances. © 1990 American Institute of Physics.
引用
收藏
页码：4750 / 4760
页数：11
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