RELAXATION PHENOMENA IN SELF-ASSEMBLED SYSTEMS

被引:8
|
作者
LEVIN, Y
MUNDY, CJ
DAWSON, KA
机构
[1] UNIV CALIF BERKELEY,DEPT CHEM,BERKELEY,CA 94720
[2] NATL UNIV IRELAND UNIV COLL DUBLIN,DEPT CHEM,DUBLIN 4,IRELAND
来源
PHYSICA A | 1993年 / 196卷 / 02期
关键词
D O I
10.1016/0378-4371(93)90599-Y
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
A dynamical model is proposed to study the evolution of the structure factor in the isotropic phase of a frustrated spin model. The study has application to the development of structure in bicontinuous microemulsions. We consider both non-conserved order parameters (NCOP) and the conserved order parameters (COP). In the former case (NCOP), within a self-consistent meanfield theory, we find that in the asymptotic limit (t --> infinity) all modes of the structure factor decay with the same characteristic time. This characteristic time scales with the two fundamental lengths d and xi is present in self-assembled systems such as frustrated magnetic systems and binary alloys. In the latter case (COP), we find that no characteristic time is present within self-consistent mean-field theory and all modes decay algebraically. This is reminiscent of the long time tails in the velocity-velocity autocorrelation function observed for simple fluids.
引用
收藏
页码:173 / 187
页数:15
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